Spectrum and low-energy gap in triangular quantum spin liquid NaYbSe$_2$

• DOI: 10.48550/arxiv.2406.17773
• Publication Date: 2024-01-01
• Authors: Scheie, A. O.; Lee, Minseong; Wang, Kevin; Laurell, P.; Choi, E. S.; Pajerowski, D.; Zhang, Qingming; Ma, Jie; Zhou, H. D.; Lee, Sangyun; Thomas, S. M.; Ajeesh, M. O.; Rosa, P. F. S.; Chen, Ao; Zapf, Vivien S.; Heyl, M.; Batista, C. D.; Dagotto, E.; Moore, J. E.; Tennant, D. Alan
• Keywords: Condensed Matter - Strongly Correlated Electrons; Strongly Correlated Electrons (cond-mat.str-el); FOS: Physical sciences

We report neutron scattering, pressure-dependent AC calorimetry, and AC magnetic susceptibility measurements of triangular lattice NaYbSe$_2$. We observe a continuum of scattering, which is reproduced by matrix product simulations, and no phase transition is detected in any bulk measurements. Comparison to heat capacity simulations suggest the material is within the Heisenberg spin liquid phase. AC Susceptibility shows a significant 23~mK downturn, indicating a gap in the magnetic spectrum. The combination of a gap with no detectable magnetic order, comparison to theoretical models, and comparison to other $A$YbSe$_2$ compounds all strongly indicate NaYbSe$_2$ is within the quantum spin liquid phase. The gap also allows us to rule out a gapless Dirac spin liquid, with a gapped $\mathbb{Z}_2$ liquid the most natural explanation.<br/>5 pages, 4 figures; 7 pages and 13 figures supplemental materials<br/>