Markus Stiller

ORCID: 0000-0003-1415-250X
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Research Areas
  • Graphene research and applications
  • Graphite, nuclear technology, radiation studies
  • Surface and Thin Film Phenomena
  • ZnO doping and properties
  • Advanced Condensed Matter Physics
  • Electronic and Structural Properties of Oxides
  • Advancements in Battery Materials
  • High-pressure geophysics and materials
  • Topological Materials and Phenomena
  • TiO2 Photocatalysis and Solar Cells
  • Chemical and Physical Properties of Materials
  • Force Microscopy Techniques and Applications
  • Magnetic properties of thin films
  • Transition Metal Oxide Nanomaterials
  • Fiber-reinforced polymer composites
  • Diamond and Carbon-based Materials Research
  • Quantum and electron transport phenomena
  • Ga2O3 and related materials
  • Advanced Photocatalysis Techniques
  • Heusler alloys: electronic and magnetic properties
  • Ion-surface interactions and analysis
  • Mechanical and Optical Resonators
  • Electrocatalysts for Energy Conversion
  • Metamaterials and Metasurfaces Applications
  • Advanced Nanomaterials in Catalysis

Leipzig University
2013-2023

Centre Marc Bloch
2019

The magnetic moment and the order induced by localized defects, like vacancies, interstitials, and/or nonmagnetic (NM) ions, in a NM oxide atomic lattice are discussed. When defect concentration is of or larger than ≈3 at%, at room temperature can appear. Herein, theoretical basic principles needed to understand compute this new phenomenon solids developed detail. In particular, main results density functional theory (DFT) calculations used estimate magnetization X‐ray circular dichroism...

10.1002/pssb.201900623 article EN cc-by physica status solidi (b) 2019-12-21

Granular superconductivity at high temperatures in graphite can emerge certain two-dimensional (2D) stacking faults (SFs) between regions with twisted (around the c-axis) or untwisted crystalline Bernal (ABA…) and/or rhombohedral (ABCABCA…) order. One way to observe experimentally such 2D is measure frozen magnetic flux produced by a permanent current loop that remains after removing an external field applied normal SFs. Magnetic force microscopy was used localize and characterize path found...

10.3390/ma15103422 article EN Materials 2022-05-10

The electrical, in-plane resistance as a function of temperature $R(T)$ bulk and mesoscopic thin graphite flakes obtained from the same batch was investigated. Samples thicker than $\ensuremath{\sim}30$ nm show metalliclike contribution in range that increases with sample thickness, whereas semiconductinglike behavior observed for thinner samples. dependence all measured samples several others literature can be very well explained between 2 1100 K assuming three contributions parallel:...

10.1103/physrevb.95.045308 article EN Physical review. B./Physical review. B 2017-01-24

Magnetic order at room temperature induced by atomic lattice defects, like vacancies, interstitials, or their pairs, has been observed in a large number of different non-magnetic hosts, such as pure graphite, oxides, and silicon-based materials. High Curie temperatures time-independent magnetic response indicate the extraordinary robustness this new phenomenon solid-state magnetism. In work, we review experimental theoretical results TiO 2 (anatase), whose can be triggered low-energy ion...

10.3389/fphy.2023.1124924 article EN cc-by Frontiers in Physics 2023-02-01

We investigated the electric transport properties of single TiO2 nanotubes separated from an anodic titania nanotube array. The temperature dependence resistance measured with conventional four point method all samples show a Mott variable range hopping behavior. results obtained two contacts indicate existence potential barrier between Cr/Au and surfaces, which influence is clearly observable at temperatures <150 K. Impedance spectroscopy in frequency 40 Hz to 1 MHz carried out room...

10.1063/1.4826640 article EN Applied Physics Letters 2013-10-21

We present a new method to obtain topological insulator Bi2Se3 thin films with centimeter large lateral length. To produce amorphous films, we have used sequential flash-evaporation at room temperature. Transmission electron microscopy has been verify that the prepared samples are in pure state. During annealing, transform into rhombohedral crystalline structure which was confirmed using X-ray diffraction and Raman spectroscopy. Resistance measurements of show expected Mott variable range...

10.1063/1.4908007 article EN Journal of Applied Physics 2015-02-17

The temperature and field dependence of the magnetization epitaxial, undoped anatase TiO2 thin films on SrTiO3 substrates was investigated. Low-energy ion irradiation used to modify surface within a few nanometers, yet with high enough energy produce oxygen titanium vacancies. as-prepared film shows ferromagnetism which increases after low-energy ions. An optimal clear magnetic anisotropy observed first irradiation, opposite expected form anisotropy. Taking into account experimental...

10.1063/1.4971794 article EN cc-by AIP Advances 2016-12-01

Abstract The magnetization of nitrogen-doped single crystalline diamond bulk samples shows unconventional field and temperature hysteresis loops at T $${\boldsymbol{\lesssim }}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mo>≲</mml:mo> </mml:math> 25 K. results suggest the existence superparamagnetic superconducting regions in with nitrogen concentration &lt;200 ppm. Both phases vanish temperatures above K where show diamagnetic behavior similar to undoped diamond....

10.1038/s41598-019-45004-6 article EN cc-by Scientific Reports 2019-06-19

In this work we have used focused electron beam induced deposition of cobalt to functionalize atomic force microscopy Akiyama tips for application in magnetic microscopy. The grown a content ≈ Co after exposure ambient air. were characterized using energy dispersive x-ray spectroscopy and scanning order investigate the properties, current loops prepared by lithography. Measurements at room temperature as well carried out coercive field mT tip was estimated applying several external fields...

10.1088/1361-6501/aa925e article EN Measurement Science and Technology 2017-10-10

This work focuses on the generation of ferromagnetism at surface anatase ${\mathrm{TiO}}_{2}$ films by low-energy ion irradiation. Controlled ${\mathrm{Ar}}^{+}$-ion irradiation resulted in a thin $(\ensuremath{\sim}10)$ nm ferromagnetic layer. The intrinsic origin and robustness magnetic order has been characterized x-ray circular dichroism room temperature revealing that Ti band is spin-polarized. These results, together with density functional theory calculations, indicate...

10.1103/physrevb.101.014412 article EN Physical review. B./Physical review. B 2020-01-09

A model identifying defects formation and structural as well chemical changes crucial parameters for a co-catalyst free photocatalytic H 2 evolution activity in epitaxial grown anatase single crystals is presented.

10.1039/d1ta04809k article EN Journal of Materials Chemistry A 2021-01-01

Tunneling atomic force microscopy (TUNA) was used at ambient conditions to measure the current-voltage $(I\text{\ensuremath{-}}V)$ characteristics clean surfaces of highly oriented graphite samples with Bernal and rhombohedral stacking orders. The characteristic curves measured on Bernal-stacked can be understood an ordinary self-consistent semiconductor modeling quantum mechanical tunneling current derivations. We show that absence a voltage region without measurable in...

10.1103/physrevmaterials.5.044601 article EN Physical Review Materials 2021-04-05

A detailed magnetoresistance (MR) study of bulk and microflake samples highly oriented pyrolytic graphite in a broad temperature $240\ensuremath{\gtrsim}T\ensuremath{\gtrsim}1\phantom{\rule{0.16em}{0ex}}\mathrm{K}$ magnetic field ${\ensuremath{\mu}}_{0}H\phantom{\rule{0.16em}{0ex}}\ensuremath{\le}62\phantom{\rule{0.16em}{0ex}}\mathrm{T}$ range, reveals the existence three independent phenomena, contributions which are observed at different temperatures fields. The identification phenomena...

10.1103/physrevmaterials.3.054603 article EN publisher-specific-oa Physical Review Materials 2019-05-17

In this work we investigated the electrical properties of rapidly quenched amorphous Bi x Sb alloys in temperature range 1.2 K to 345 K. The resistance reveals that for a broad different compositions, including topological insulator (TI), superconducting state phase is present. After crystallization and annealing at an intermediate temperature, found pure with composition corresponding TI, superconductivity persists, but transition shifts lower temperature. highest was those TI's, shift low...

10.1088/0953-2048/30/1/015013 article EN Superconductor Science and Technology 2016-11-15

We have investigated the electrical resistance R(T) of ZnO nanowires ≈ 400 nm diameter as a function temperature, between 30 K and 300 K, frequency in range 40 Hz to MHz. The measurements were done on as-prepared after low-energy proton implantation at room temperature. temperature dependence wire, before implantation, can be well described by two processes parallel. One process is fluctuation induced tunneling conductance (FITC) other usual thermally activated process. existence was also...

10.1088/0957-4484/26/39/395703 article EN Nanotechnology 2015-09-11

We report measurements of transmission electron microscopy, the electrical resistivity, magnetoresistance and Hall effect (HE) in amorphous quasicrystalline (QC) phase . The samples are prepared situ at K as thin films phase. After preparation, sample was measured during annealing different temperatures. were performed temperature range 1.2–300 with fields up to ±8 T. Atomic structure information obtained by spectroscopy reveals that icosahedral local atomic order is already present improved...

10.1088/2053-1591/2/9/096403 article EN Materials Research Express 2015-09-10

Granular superconductivity at high temperatures in graphite can emerge certain two-dimensional (2D) stacking faults (SFs) between regions with twisted (around the c-axis) or untwisted crystalline Bernal (ABA...) and/or rhombohedral (ABCABCA...) order. One way to observe experimentally such 2D is measure frozen magnetic flux produced by a permanent current loop that remains after removing an external field applied normal SFs. Magnetic force microscopy was used localize and characterize path...

10.20944/preprints202204.0209.v1 preprint EN 2022-04-22

Placing electrodes at the edges of stacking faults, for example between Bernal and rhombohedral orders as in sketch, observable by transmission electron microscopy a micrometer-size Sri Lankan natural graphite sample, record values change resistance with magnetic field has been found. The magnetoresistance (MR) increases linearly reaches ≈107% B = 21 T. For more details please refer to article Pablo D. Esquinazi co-workers number 1900991.

10.1002/adem.201970039 article EN Advanced Engineering Materials 2019-12-01
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