Jacqueline Edge

ORCID: 0000-0003-4643-2426
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About
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Research Areas
  • Advancements in Battery Materials
  • Advanced Battery Technologies Research
  • Extraction and Separation Processes
  • Advanced Battery Materials and Technologies
  • Recycling and Waste Management Techniques
  • Electric Vehicles and Infrastructure
  • Environmental Impact and Sustainability
  • Hydrogen Storage and Materials
  • Innovative Energy Harvesting Technologies
  • Advanced DC-DC Converters
  • Phase Equilibria and Thermodynamics
  • Semiconductor Quantum Structures and Devices
  • NMR spectroscopy and applications
  • Field-Flow Fractionation Techniques
  • GaN-based semiconductor devices and materials
  • Quantum, superfluid, helium dynamics
  • Advancements in Solid Oxide Fuel Cells
  • Thermodynamic properties of mixtures
  • Acoustic Wave Resonator Technologies
  • Green IT and Sustainability
  • Soil and Unsaturated Flow
  • Mining and Resource Management
  • Chemical and Physical Properties in Aqueous Solutions
  • Carbon Dioxide Capture Technologies
  • Hydrogen embrittlement and corrosion behaviors in metals

The Faraday Institution
2021-2024

Imperial College London
1997-2024

Research Network (United States)
2017

London Centre for Nanotechnology
2012-2014

University College London
2012

Australian National University
2006

The expansion of lithium-ion batteries from consumer electronics to larger-scale transport and energy storage applications has made understanding the many mechanisms responsible for battery degradation increasingly important.

10.1039/d1cp00359c article EN cc-by Physical Chemistry Chemical Physics 2021-01-01

Economically viable electric vehicle lithium-ion battery recycling is increasingly needed; however routes to profitability are still unclear. We present a comprehensive, holistic techno-economic model as framework directly compare locations and processes, providing key tool for cost optimization in an international economy. show that can be economically viable, with cost/profit ranging from (−21.43 - +21.91) $·kWh−1 but strongly depends on transport distances, wages, pack design method....

10.1016/j.isci.2021.102787 article EN cc-by iScience 2021-06-26

Predicting lithium-ion battery degradation is worth billions to the global automotive, aviation and energy storage industries, improve performance safety reduce warranty liabilities. However, very few published models of explicitly consider interactions between more than two mechanisms, none do so within a single electrode. In this paper, first attempt directly couple mechanisms in negative electrode reported. The results are used map different pathways through complicated path dependent...

10.1039/d2cp00417h article EN cc-by Physical Chemistry Chemical Physics 2022-01-01

Abstract Physics-based electrochemical battery models derived from porous electrode theory are a very powerful tool for understanding lithium-ion batteries, as well improving their design and management. Different model fidelity, thus complexity, is needed different applications. For example, in we can afford longer computational times the use of computers, while real-time control (e.g. electric vehicles) need to perform fast calculations using simple devices. this reason, simplified that...

10.1088/2516-1083/ac7d31 article EN cc-by Progress in Energy 2022-06-29

Abstract The market dynamics, and their impact on a future circular economy for lithium-ion batteries (LIB), are presented in this roadmap, with safety as an integral consideration throughout the life cycle. At point of end-of-life (EOL), there is range potential options—remanufacturing, reuse recycling. Diagnostics play significant role evaluating state-of-health condition batteries, improvements to diagnostic techniques evaluated. present, manual disassembly dominates EOL disposal,...

10.1088/2515-7655/acaa57 article EN cc-by Journal of Physics Energy 2022-12-09

Abstract The heavy reliance of lithium-ion batteries (LIBs) has caused rising concerns on the sustainability lithium and transition metal ethic issue around mining practice. Developing alternative energy storage technologies beyond become a prominent slice global research portfolio. play vital role in shaping future landscape storage, from electrified mobility to efficient utilization renewable energies further large-scale stationary storage. Potassium-ion (PIBs) are promising given its...

10.1088/2515-7655/acbf76 article EN cc-by Journal of Physics Energy 2023-02-27

The pursuit of low-carbon transport has significantly increased demand for lithium-ion batteries. However, the rapid increase in battery manufacturing, without adequate consideration carbon emissions associated with their production and material demands, poses threat shifting bulk upstream. In this article, a life cycle assessment (LCA) model is developed to account cradle-to-gate footprint batteries across 26 Chinese provinces, 20 North American locations 19 countries Europe Asia. Analysis...

10.1016/j.jclepro.2024.141725 article EN cc-by Journal of Cleaner Production 2024-03-09

The electrification of the transport sector is a critical part net-zero transition. mass adoption electric vehicles (EVs) powered by lithium-ion batteries in coming decade will inevitably lead to large amount battery waste, which needs handling safe and environmentally friendly manner. Battery recycling sustainable treatment option at end-of-life that supports circular economy. However, heterogeneity pack designs across manufacturers are hampering establishment an efficient disassembly...

10.1016/j.apenergy.2022.120437 article EN cc-by Applied Energy 2022-12-05

The Doyle-Fuller-Newman framework is the most popular physics-based continuum-level description of chemical and dynamical internal processes within operating lithium-ion-battery cells. With sufficient flexibility to model a wide range battery designs chemistries, provides an effective balance between detail, needed capture key microscopic mechanisms, simplicity, solve governing equations at relatively modest computational expense. Nevertheless, implementation requires values numerous...

10.1088/2516-1083/ac692c article EN cc-by Progress in Energy 2022-04-21

While electric vehicles are seen as an important tool in the decarbonisation of transport, pack and module architectures make disassembly recycling slow complex. Removal physical fastenings such clips, screws, welds adhesives rate limiting factor to cell disassembly. This study investigates types polymeric which used various battery components shows how careful choice can speed up circumvent need for shredding increase purity value recycled material.

10.1016/j.nxener.2023.100023 article EN cc-by Next Energy 2023-05-20

Net zero targets have resulted in a drive to decarbonise the transport sector worldwide through electrification. This has, turn, led an exponentially growing battery market and, conversely, increasing attention on how we can reduce environmental impact of batteries and promote more efficient circular economy achieve real net zero. As these reach end their first life, challenges arise as collect process them, order maximise economical use before finally being recycled. Despite body work...

10.3389/fchem.2024.1358417 article EN cc-by Frontiers in Chemistry 2024-04-08

Abstract With the number of electric vehicles (EVs) projected to increase 25‐fold by 2030, effective recycling processes need be developed conserve critical raw materials (in particular, cobalt and lithium) used make lithium‐ion batteries (LIBs). Industrial LIBs is underdeveloped due two main reasons: i) complex particularly variable cathodic chemistries; ii) physically different shapes sizes battery packs which are not designed for easy disassembly. Present use pyrometallurgical and/or...

10.1002/batt.202000146 article EN Batteries & Supercaps 2020-07-22

Abstract Computational modelling is a vital tool in the research of batteries and their component materials. Atomistic models are key to building truly physics-based form foundation multiscale chain, leading more robust predictive models. These can be applied fundamental questions with high accuracy. For example, they used predict new behaviour not currently accessible by experiment, for reasons cost, safety, or throughput. useful quantifying evaluating trends experimental data, explaining...

10.1088/2516-1083/ac3894 article EN cc-by Progress in Energy 2021-11-10

First-generation cathodes for commercial lithium-ion batteries are based on layered transition-metal oxides. Research ternary compounds, such as LiCoO2, evolved into mixed-metal systems, notably Li(Ni,Mn,Co)O2 (NMCs), which allows significant tuning of the physical properties. Despite their widespread application in devices, fundamental understanding NMCs is incomplete. Here, we review latest insights from multiscale modeling, bridging between redox phenomena that occur at an atomistic level...

10.1021/acsenergylett.1c02028 article EN ACS Energy Letters 2021-12-03

Abstract The transition towards renewable energy and electric transportation depends on the development of efficient storage technologies. Lithium‐ion batteries (LIBs) have gained increasing popularity despite rising prices uncertainty around sourcing component materials. This has recently prompted alternative alkali batteries, such as sodium‐ion (SIBs). However, academic efforts focused optimizing technical performance, few studied underlying economic environmental impacts batteries....

10.1002/adsu.202200047 article EN Advanced Sustainable Systems 2022-04-11

Many of the issues associated with recycling devices containing small but significant amounts technology critical metals, arise from choice materials and, most importantly, joining methods for...

10.1039/d5su00128e article EN cc-by RSC Sustainability 2025-01-01

IOP journal sustainability science and technology (sus sci tech) in 2024 beyond: equitable publishing aligned with United Nations' sustainable development goals (SDGs), Jonas Baltrusaitis, Bhavik Bakashi, Katarzyna Chojnacka, Christopher Chuck, Marc-Olivier Coppens, Jacqueline Sophie Edge, Gavin Harper, Benjamin Hsiao, Hao Li, Mark Mba-Wright, Michael McLaughlin, Arpita Nandy, Shu-Yuan Pan (潘述元), Zhe Qiang, Cauê Ribeiro de Oliveira, Malgorzata Swadzba-Kwasny, Meng Wang, Yizhi Xiang, Lizhi Zhang

10.1088/2977-3504/ad555a article EN cc-by Deleted Journal 2024-06-07

Neutron scattering has been used to reveal the structure and dynamics of molecular H2 physisorbed into two-dimensional pores sparingly hydrated Ca-laponite clay. Thermal pretreatment clay at 415 K under vacuum yielded an interlayer composition in 1.0–1.5 water molecules per Ca2+ cation range provided a vacant gallery height 2.82 Å. This value is very well matched diameter hydrogen allows intercalation up point where liquid-like monolayer formed within At low coverage 0.1 isosteric heat...

10.1021/jp5082356 article EN The Journal of Physical Chemistry C 2014-10-11

Abstract Invited for this month's cover picture is the group of Electrochemical Science and Engineering at Imperial College London including Titirici Group. The shows a schematic illustration batteries recycling. Read full text Review 10.1002/batt.202000146 .

10.1002/batt.202000231 article EN Batteries & Supercaps 2020-10-19

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTEffects of proton exchange on diffusion in aqueous solutions methanolAllan J. Easteal, A. Vernon, Edge, and Lawrence WoolfCite this: Phys. Chem. 1985, 89, 7, 1064–1066Publication Date (Print):March 1, 1985Publication History Published online1 May 2002Published inissue 1 March 1985https://pubs.acs.org/doi/10.1021/j100253a003https://doi.org/10.1021/j100253a003research-articleACS PublicationsRequest reuse permissionsArticle...

10.1021/j100253a003 article EN The Journal of Physical Chemistry 1985-03-01

Abstract Electric vehicles using lithium-ion batteries are currently the most promising technology to decarbonise transport sector from fossil-fuels. It is thus imperative reduce battery life cycle costs and greenhouse gas emissions make this transition both economically environmentally beneficial. In study, it shown that lifetime extension through effective thermal management significantly decreases cost carbon footprint. The simulated for each system implemented in techno-economic...

10.1149/ma2021-0222743mtgabs article EN Meeting abstracts/Meeting abstracts (Electrochemical Society. CD-ROM) 2021-10-19

10.1595/205651317x695839 article EN cc-by Johnson Matthey Technology Review 2017-07-01
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