Fabricated Biobased Eucommia Ulmoides Gum/Polyolefin Elastomer Thermoplastic Vulcanizates into a Shape Memory Material
Polyolefin
Thermoplastic elastomer
DOI:
10.1021/acs.iecr.8b04710
Publication Date:
2019-04-08T14:44:33Z
AUTHORS (7)
ABSTRACT
Partially biobased thermoplastic vulcanizates (TPVs) with shape memory properties were prepared by in situ dynamic vulcanization of eucommia ulmoides gum (EUG) and polyolefin elastomer (POE). The cross-linked EUG phase dispersed POE matrix acted as a framework structure throughout the phase, which limited irreversible deformation provided sufficient resilience force to drive molecular chains recover their initial shape. results demonstrated that EUG/POE TPVs exhibited excellent high fixity recovery rate (all above 95%). dimensions 0.4–1.6 μm matrix, more resulted large aggregates. considerably improved permanent POE, tensile set linearly decreases from 134% 4% increasing contents. mechanical changed little after being reprocessed twice, exhibiting good reprocessability. All these remarkable advantages make candidates for materials.
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