Constraining calculations of Pu239(n,γ) cross sections with multistep cascade γ -ray spectra measured at the DANCE facility

• DOI: 10.1103/physrevc.111.024610
• Publication Date: 2025-02-13T16:19:23Z
• Authors: J. L. Ullmann; T. Kawano; B. Baramsai; T. A. Bredeweg; A. Couture; M. Jandel; S. Mosby; J. M. O'Donnell; R. S. Rundberg; H. Sasaki; D. J. Vieira; J. B. Wilhelmy; M. Krtička; A. Chyzh; R. Henderson; C. Y. Wu

Measurements of multistep cascade gamma-ray spectra from several low-lying 1+ resonances in the Pu239(n,γ) reaction were made using the DANCE detector. The measured spectra are compared to spectra simulated using several models for the photon strength function and the nuclear level density, representing the first analysis of this nature on a fissile nucleus. In general, models of the photon strength function that included a strong M1 “scissors mode” contribution coupled with a Gilbert-Cameron nuclear level density provided a reasonable description of the spectra. Simulations using photon strength functions and nuclear level densities specifically for Pu240, extracted by the Oslo method, resulted in a very good representation of the measured spectra. Neutron-capture cross section calculations that included the scissors mode provided a good estimate of the previously measured values, without additional normalization. However, the scissors-mode energy that produced the best description of the multistep cascade spectra was different from the value that best reproduced the capture cross section. In addition, the 〈Γγ〉 inferred from the multistep cascade calculations was somewhat less than the tabulated value, which was determined from resonance analysis.

Published by the American Physical Society 2025