Yajie Song

ORCID: 0009-0009-0238-9383
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Research Areas
  • Advancements in Battery Materials
  • Advanced Battery Materials and Technologies
  • Advanced Battery Technologies Research
  • Advanced battery technologies research
  • Electrocatalysts for Energy Conversion
  • Crystallization and Solubility Studies
  • Supercapacitor Materials and Fabrication
  • Hydrogen Storage and Materials
  • X-ray Diffraction in Crystallography
  • Fuel Cells and Related Materials
  • Ammonia Synthesis and Nitrogen Reduction
  • Electrochemical Analysis and Applications
  • Catalytic Processes in Materials Science
  • Layered Double Hydroxides Synthesis and Applications
  • Soil Carbon and Nitrogen Dynamics
  • Lanthanide and Transition Metal Complexes
  • Extraction and Separation Processes
  • Electron and X-Ray Spectroscopy Techniques
  • Surface Modification and Superhydrophobicity
  • Chemical Synthesis and Characterization
  • Electrochemical sensors and biosensors
  • Polysaccharides Composition and Applications
  • Superconductivity in MgB2 and Alloys
  • Microplastics and Plastic Pollution
  • Advanced Electron Microscopy Techniques and Applications

Zhejiang University
2025

State Key Laboratory of Clean Energy Utilization
2025

South China University of Technology
1998-2025

Harbin Institute of Technology
2009-2024

Intelligent Energy (United Kingdom)
2024

Qingdao Institute of Bioenergy and Bioprocess Technology
2024

Qinghai New Energy (China)
2024

Chinese Academy of Sciences
2009-2024

Dalian University of Technology
2021-2022

Dalian University
2021

Single-atom catalysts have been paid more attention to improving sluggish reaction kinetics and anchoring polysulfide for lithium-sulfur (Li-S) batteries. It has demonstrated that d-block single-atom elements in the fourth period can chemically interact with local environment, leading effective adsorption catalytic activity toward lithium polysulfides. Enlightened by theoretical screening, first time, we design novel Nb improved sulfur immobilization catalyzation. Calculations reveal Nb-N4...

10.1021/jacs.2c10345 article EN Journal of the American Chemical Society 2023-01-14

Single atom tailored metal nanoparticles represent a new type of catalysts. Herein, we demonstrate single atom-cavity coupling strategy to regulate performance nano-catalysts. Selective atomic layer deposition (ALD) was conducted deposit Ru atoms on the surface concavities PtNi (Ru-ca-PtNi). Ru-ca-PtNi exhibits record-high activity for methanol oxidation reaction (MOR) with 2.01 A mg-1Pt . Also, showcases significant durability only 16 % loss. Operando electrochemical Fourier transform...

10.1002/anie.202207524 article EN Angewandte Chemie International Edition 2022-08-30

Owing to high ionic conductivity and mechanical strength, poly(vinylidene fluoride) (PVDF) electrolytes have attracted increasing attention for solid-state lithium batteries, but highly reactive residual solvents severely plague cycling stability. Herein, we report a free-solvent-capturing strategy triggered by reinforced ion-dipole interactions between Li+ solvent molecules. Lithium difluoro(oxalato)borate (LiDFOB) salt additive with electron-withdrawing capability serves as redistributor...

10.1021/jacs.3c07482 article EN Journal of the American Chemical Society 2023-11-09

Polyethylene oxide (PEO) based electrolytes critically govern the security and energy density of solid-state batteries, but typically suffer from poor oxidation resistance at high voltages, which limits batteries. Here, we report a Lewis-acid coordinated strategy to significantly improve cyclic stability 4.8 V-class PEO-based battery. The introduced Mg

10.1038/s41467-024-53094-8 article EN cc-by-nc-nd Nature Communications 2024-10-23

Abstract The interfacial stability between sulfide solid‐state electrolytes (SSEs) and high voltage Ni‐rich oxide cathodes is critical to the electrochemical performances of all‐solid‐state batteries (ASSBs), yet it challenging solve interface issues by surface coating modification. Here, a surface‐to‐bulk synergistic modification proposed achieve highly stable through combination TiNb 2 O 7 ‐coated Ti‐doped LiNi 0.6 Mn 0.2 Co single crystals (DC‐TNO@SCNCM). layer with...

10.1002/aenm.202200682 article EN Advanced Energy Materials 2022-06-17

Abstract The complicated interfacial problems of poly(ethylene oxide) (PEO)‐based solid polymer electrolytes (SPEs) at high voltages severely hinder its practical applications for high‐energy‐density all‐solid‐state lithium batteries (ASSLBs). Herein, the failure mechanisms ASSLBs with LiNi 0.6 Co 0.2 Mn O 2 (NCM)‐PEO are studied. It is found that after charge generates a sharp drop 0.62 V cut‐off voltage 4.30 V, and induce resistance due to forming an uneven thick cathode electrolyte...

10.1002/adfm.202113068 article EN Advanced Functional Materials 2022-03-01

All-solid-state batteries (ASSBs) have attracted considerable attention due to their theoretically high energy density and safety. However, maintaining intimate interfacial contact at low external pressures remains a challenge, limiting large-scale practical applications. Here, bottom-up design of all-solid-state electrodes is proposed by minimizing internal stress variation maintain transport pressures. Theoretical calculations synchrotron X-ray techniques reveal that the surface-to-bulk...

10.1021/acsenergylett.3c01840 article EN ACS Energy Letters 2023-11-07

Solid-state Li-O 2 batteries (SSLOBs) have attracted considerable attention because of their high energy density and superior safety. However, sluggish kinetics severely impeded practical application. Despite efforts to design highly efficient catalysts, oxygen reaction evolution at gas-solid interfaces fast transport pathways in solid-state electrodes remain challenging. Here, we develop a dual electronic-ionic microenvironment substantially enhance electrolysis batteries. By designing...

10.1126/sciadv.abq6261 article EN cc-by-nc Science Advances 2022-09-02

Superparamagnetic iron oxide nanoparticles (SPION) are potential drug carriers and a magnetic resonance imaging (MRI) contrast agent for cancer therapy diagnosis. In this study, dechlorinated cisplatin (CMDP) is tethered to maghemite modified with 4-oxo-4-(3-(triethoxysilyl)propylamino)butanoic acid (OTPBA–SPION) through the surface carboxylate groups. The nanocomposite (CMDP–OTPBA–SPION) was characterized by TEM, XPS, EDX, SQUID, ICP-AES, zeta potential. A relatively high Pt loading...

10.1039/c3sc50554e article EN Chemical Science 2013-01-01

Plastic fragments are widely found in the soil profile of terrestrial ecosystems, forming plastic footprint and posing increasing threat to functionality carbon (C) footprint. It is unclear how affects C cycling, particularly permanent sequestration. Integrated field observations (including 13C labelling) were made using polyethylene polylactic acid (low-, medium- high-concentrations as intensifying footprint) landfilling soil, track flow along soil–plant-atmosphere continuum (SPAC). The...

10.1016/j.envint.2024.108632 article EN cc-by-nc-nd Environment International 2024-04-01

Two monofunctional platinum(II) complexes, cis-[PtL(NH3)2Cl]NO3 (1) and cis-[PtL′(NH3)2Cl]NO3 (2) {L = N-methyl-7-nitro-N-(2-(pyridin-2-yl)ethyl)benzo[c][1,2,5]-oxadiazol-4-amine, L′ 7-nitro-N-(2-(pyridin-2-yl)ethyl)benzo[c][1,2,5] oxadiazol-4-amine}, have been synthesized characterized. The X-ray single crystal structure of complex 1 shows that is coordinated in a square-planar geometry with [PtN3Cl] setting. Fluorescence profiles the complexes show more suitable for cellular imaging than...

10.1039/c1dt10555h article EN Dalton Transactions 2011-01-01

Abstract Solid‐state lithium‐oxygen batteries (SSLOBs) offer high energy density with enhanced safety. However, the challenge of loss induced by polarization solid‐state air electrode has become a major bottleneck for its further development. Here, homonuclear Fe‐Fe catalyst (Fe 2 ‐N‐C) matched to reactants (Li 2‐x O , 0 ≤ x 2) size alleviate redox in electrodes is designed. Atomically resolved transmission electron microscopy reveals that spatial clusters (1.5–2 Å) commensurate Li (1.2–2.2...

10.1002/aenm.202203660 article EN Advanced Energy Materials 2022-12-08

Dynamic interactions of the droplet impact on a solid surface are essential to many emerging applications, such as electronics cooling, ink-jet printing, water harvesting/collection, anti-frosting/icing, and microfluidic biomedical device applications. Despite extensive studies kinematic features over last two decades, spreading characteristics hydrophilic with ultra-low contact angle hysteresis unclear. This paper clarifies specific role at each stage process. The an ultra-slippery...

10.3390/coatings12060755 article EN Coatings 2022-05-31
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