Tiefeng Liu

ORCID: 0000-0001-7251-624X
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About
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Research Areas
  • Conducting polymers and applications
  • Organic Electronics and Photovoltaics
  • Perovskite Materials and Applications
  • Advanced Sensor and Energy Harvesting Materials
  • Chalcogenide Semiconductor Thin Films
  • Supercapacitor Materials and Fabrication
  • Organic Light-Emitting Diodes Research
  • Quantum Dots Synthesis And Properties
  • Advanced Battery Materials and Technologies
  • Advancements in Battery Materials
  • Semiconductor materials and interfaces
  • Advanced Thermoelectric Materials and Devices
  • Analytical Chemistry and Sensors
  • Advanced Memory and Neural Computing
  • Thermochemical Biomass Conversion Processes
  • Advanced battery technologies research
  • Coal and Its By-products
  • Advanced Battery Technologies Research
  • Nanomaterials and Printing Technologies
  • solar cell performance optimization
  • Ionic liquids properties and applications
  • Fuel Cells and Related Materials
  • Thin-Film Transistor Technologies
  • Chemistry and Chemical Engineering
  • Electrocatalysts for Energy Conversion

Zhejiang University
2025

Linköping University
2023-2024

Wallenberg Wood Science Center
2024

Chung-Ang University
2024

Wuhan National Laboratory for Optoelectronics
2015-2022

Huazhong University of Science and Technology
2015-2022

Optica
2018

Institute of Coal Chemistry
2008

University of Chinese Academy of Sciences
2008

The environmental toxicity of Pb in organic–inorganic hybrid perovskite solar cells remains an issue, which has triggered intense research on seeking alternative Pb-free perovskites for applications. Halide based group-VA cations Bi3+ and Sb3+ with the same lone-pair ns2 state as Pb2+ are promising candidates. Herein, through a joint experimental theoretical study, we demonstrate that Cl-incorporated methylammonium Sb halide (CH3NH3)3Sb2ClXI9–X show promise efficient absorbers cells....

10.1021/jacs.7b10739 article EN Journal of the American Chemical Society 2017-12-23

Nonfullerene acceptors tend to decompose in the presence of ZnO due photocatalytic activity, and SnO<sub>2</sub>is an alternative for higher efficiency better stability.

10.1039/c9mh00379g article EN Materials Horizons 2019-01-01

Achieving high power conversion efficiency and good mechanical robustness is still challenging for the ultraflexible organic solar cells. Interlayers simultaneously having chemical compatibility with active layer are highly desirable. In this work, we present an interlayer of Zn2+-chelated polyethylenimine (denoted as PEI-Zn), which can endure a maximum bending strain over twice that ZnO chemically compatible recently emerging efficient nonfullerene layers. On 1.3 μm polyethylene naphthalate...

10.1038/s41467-020-18373-0 article EN cc-by Nature Communications 2020-09-09

All-solution-processed organic solar cells (from the bottom substrate to top electrode) are highly desirable for low-cost and ubiquitous applications. However, it is still challenging fabricate efficient all-solution-processed with a high-performance nonfullerene (NF) active layer. Issues of charge extraction wetting persistent at interface between layer printable electrode (PEDOT:PSS). In this work, NF reported via adoption hydrogen molybdenum bronze (HX MoO3 ) PEDOT:PSS. The dual functions...

10.1002/adma.201907840 article EN Advanced Materials 2020-02-24

Abstract Poly(3,4‐ethylenedioxythiophene) (PEDOT) is a very unique polymer. It can be conductive, highly transparent, and environmentally stable. switchable between its oxidation state neutral state. forms micellar complex with polystyrene sulfonate in aqueous conditions, then solution‐processible printable. Based on these advantages, PEDOT has been widely used as conductors transparent electrodes electronics optoelectronics. The device performance correlated the structure properties of...

10.1002/adfm.202006213 article EN Advanced Functional Materials 2020-09-16

Abstract Development of large‐area flexible organic solar cells (OSCs) is highly desirable for their practical applications. However, the efficiency OSCs severely lags behind small‐area devices. Here, efficient single with power conversion (PCE) 13.1% and 12.6% areas 6 10 cm 2 , modules a PCE 13.2% (54 ) based on poly(ethylene terephthalate)/Ag grid/silver nanowires (AgNWs):zinc‐chelated polyethylenimine (PEI‐Zn) composite electrodes are reported. The solution‐processed transparent electrode...

10.1002/adma.202103017 article EN Advanced Materials 2021-08-08

Abstract Chemical doping is an important approach to manipulating charge-carrier concentration and transport in organic semiconductors (OSCs) 1–3 ultimately enhances device performance 4–7 . However, conventional strategies often rely on the use of highly reactive (strong) dopants 8–10 , which are consumed during process. Achieving efficient with weak and/or widely accessible under mild conditions remains a considerable challenge. Here, we report previously undescribed concept for...

10.1038/s41586-024-07400-5 article EN cc-by Nature 2024-05-15

The first bottom-up solution-processed perovskite–perovskite tandem solar cell has been successfully fabricated <italic>via</italic> an optimized charge recombination layer comprising spiro-OMeTAD/PEDOT:PSS/PEI/PCBM:PEI. as-fabricated device delivers open voltage of up to 1.89 V, close the sum two perovskite subcells.

10.1039/c5ta08744a article EN Journal of Materials Chemistry A 2015-12-15

Abstract Thick, uniform, easily processed, highly conductive polymer films are desirable as electrodes for solar cells well capacitors. Here, a novel scalable strategy is developed to prepare thick poly(3,4‐ethylenedioxythiophene):polystyrene sulfonate (HCT‐PEDOT:PSS) with layered structure that display conductivity of 1400 S cm −1 and low sheet resistance 0.59 ohm sq . Organic laminated HCT‐PEDOT:PSS exhibit performance comparable the reference devices vacuum‐deposited Ag top electrodes....

10.1002/anie.201509033 article EN Angewandte Chemie International Edition 2015-12-02

Abstract Binder plays a key role in maintaining the mechanical integrity of electrodes lithium‐ion batteries. However, existing binders typically exhibit poor stretchability or low conductivity at large strains, which are not suitable for high‐capacity silicon (Si)‐based anodes undergoing severe volume changes during cycling. Herein, novel stretchable conductive glue (CG) polymer that possesses inherent high conductivity, excellent stretchablity, and ductility is designed high‐performance Si...

10.1002/adfm.201704858 article EN Advanced Functional Materials 2017-11-27

Vertical phase distribution plays an important role in the quasi-two-dimensional perovskite solar cells. So far, driving force and how to tailor vertical of layer numbers have been not discussed. In this work, we report that films deposited on a hole-transporting is different from glass substrate. The could be explained by sedimentation equilibrium because colloidal feature precursors. Acid addition will change precursors colloid solution therefore changes distribution. A self-assembly used...

10.1038/s41467-019-08843-5 article EN cc-by Nature Communications 2019-02-20

Organometal halide perovskites have shown excellent optoelectronic properties and been used to demonstrate a variety of semiconductor devices. Colorful solar cells are desirable for photovoltaic integration in buildings other aesthetically appealing applications. However, the realization colorful perovskite is challenging because their broad large absorption coefficient that commonly leads with dark-brown colors. Herein, first time, we report simple efficient strategy achieve by using...

10.1021/acs.nanolett.6b04019 article EN Nano Letters 2016-11-23

Highly conductive polymer films on plastic substrates are desirable for the application of flexible electronics. Here, we report conductivity poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PSS) can be enhanced to 1460 S/cm via phosphoric acid (H3PO4) treatment. The enhancement is associated with partial removal PSS from film. H3PO4 treatment compatible substrates, while sulfuric (H2SO4) easily damage substrate. With electrode poly(ether sulfone) (PES)/H3PO4-treatedPSS, have...

10.1021/acsami.5b03309 article EN ACS Applied Materials & Interfaces 2015-06-08

Flexible non-fullerene organic solar cells based on AgNWs embedded in polyimide substrates demonstrate a high efficiency up to 11.6%.

10.1039/c8ta11378e article EN Journal of Materials Chemistry A 2019-01-01

Enhancing open‐circuit voltage in CH 3 NH PbI (Cl) perovskite solar cells has become a major challenge for approaching the theoretical limit of power conversion efficiency. Here, first time, it is demonstrated that synergistic effect 2 passivation and chlorine incorporation via controlling molar ratio , PbCl (or MACl), MAI precursor solutions, boosts over 1.15 V both mesoscopic inverted planar cells. Such high can be attributed to enhanced photoluminescence emission carrier lifetime...

10.1002/adfm.201603968 article EN Advanced Functional Materials 2016-09-26

Abstract Operational stability is essential for the success of organic electrochemical transistors (OECTs) in bioelectronics. The oxygen reduction reaction (ORR) a common side that can compromise OECTs, but relationship between ORR and materials degradation poorly understood. In this study, impact on mechanisms thiophene‐based OECTs investigated. findings show an increase pH during leads to polymer backbone. By using protective glue layer semiconductor channel aqueous electrolyte,...

10.1002/adfm.202302249 article EN cc-by Advanced Functional Materials 2023-06-15

Organic electrochemical transistors (OECTs) are a rapidly advancing technology that plays crucial role in the development of next-generation bioelectronic devices. Recent advances p-type/n-type organic mixed ionic-electronic conductors (OMIECs) have enabled power-efficient complementary OECT technologies for various applications, such as chemical/biological sensing, large-scale logic gates, and neuromorphic computing. However, ensuring long-term operational stability remains significant...

10.1039/d3mh00858d article EN cc-by Materials Horizons 2023-01-01

Poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) is a benchmark hole-transporting (p-type) polymer that finds applications in diverse electronic devices. Most of its success due to facile synthesis water, exceptional processability from aqueous solutions, and outstanding electrical performance ambient. Applications fields like (opto-)electronics, bioelectronics, energy harvesting/storage devices often necessitate the complementary use both p-type n-type...

10.1021/jacs.4c02270 article EN cc-by Journal of the American Chemical Society 2024-05-30

Electron and hole transport layers have critical impacts on the overall performance of perovskite solar cells (PSCs). Herein, for first time, a solution-processed cobalt (Co)-doped NiOX film was fabricated as layer in inverted planar PSCs, exhibit 18.6% power conversion efficiency. It has been found that an appropriate Co-doping can significantly adjust work function enhance electrical conductivity film. Capacitance–voltage (C–V) spectra time-resolved photoluminescence indicate clearly...

10.1021/acsami.8b01683 article EN ACS Applied Materials & Interfaces 2018-04-05

Flexible all-plastic multijunction solar cells with high photovoltage have been demonstrated <italic>via</italic> optimization of the charge-recombination layer and shown to power portable electronics.

10.1039/c6mh00164e article EN Materials Horizons 2016-01-01

Layered Ruddlesden–Popper (RP) perovskites have good moisture- and photostability. However, thermal stability of the RP is still a challenge. In this work, through joint theoretical experimental study, we report an intralayer A-site compositional engineering strategy to enhance perovskite solar cells. The triple-A-site-cation BA2(MA0.76FA0.19Cs0.05)3Pb4I13 (labeled as T-RP) cells retain 80% initial efficiency after being stressed at constant temperature 85 °C for over 1400 h in dark, which...

10.1021/acsenergylett.9b00403 article EN ACS Energy Letters 2019-05-02

Organic–inorganic hybrid perovskite solar cells have attracted great attention due to their unique properties and rapid increased power conversion efficiency. Currently, PC61BM is widely used as the electron transport layer (ETL) for inverted perovksite cells. Here we propose demonstrate that Bi2S3, a ribboned compound with intrinsic high mobility stability, could be ETL Through simple thermal evaporation substrate kept at room temperature, successfully produced compact smooth amorphous...

10.1021/acsphotonics.6b00582 article EN ACS Photonics 2016-10-12

Solution-processable poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) is a widely used hole transporting layer (HTL) in organic solar cells (OSCs). However, it challenge to adopt as the HTL on hydrophobic active layers fabricate inverted OSCs. Surfactants are generally added improve wettability of aqueous PEDOT:PSS. In this work, we report that surfactants could induce change work function (WF) PEDOT:PSS and significantly influence device performance. Fluorine-containing...

10.1021/acsaem.2c00217 article EN ACS Applied Energy Materials 2022-03-08
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