- Advanced Photocatalysis Techniques
- TiO2 Photocatalysis and Solar Cells
- Catalytic Processes in Materials Science
- Supercapacitor Materials and Fabrication
- Quantum Dots Synthesis And Properties
- Copper-based nanomaterials and applications
- Perovskite Materials and Applications
- X-ray Diffraction in Crystallography
- Crystallization and Solubility Studies
- Electrocatalysts for Energy Conversion
- Advancements in Battery Materials
- Advanced battery technologies research
- Conducting polymers and applications
- Nanomaterials for catalytic reactions
- Advanced Battery Materials and Technologies
- Advanced Nanomaterials in Catalysis
- Gas Sensing Nanomaterials and Sensors
- Ammonia Synthesis and Nitrogen Reduction
- Mesoporous Materials and Catalysis
- Metal-Organic Frameworks: Synthesis and Applications
- Crystallography and molecular interactions
- ZnO doping and properties
- Advanced oxidation water treatment
- Polyoxometalates: Synthesis and Applications
- Fuel Cells and Related Materials
Wuhan University of Technology
2022-2025
Tianjin University of Technology
2013-2025
Yanshan University
2024
State Key Laboratory of Metastable Materials Science and Technology
2024
Sichuan Normal University
2022-2023
Anhui University of Science and Technology
2023
Institute of New Materials
2023
Jiangsu University
2023
Sun Yat-sen University
2023
Science and Technology Department of Sichuan Province
2022-2023
CdS and Ni-doped hollow spheres were synthesized via a simple template-free one-pot method. The products characterized by X-ray powder diffraction, scanning electron microscopy, transmission high-resolution energy-dispersive spectroscopy analysis, photoelectron spectroscopy, UV-vis absorption spectroscopy. formation mechanism for the was discussed. prepared showed superior photocatalytic activity degradation of RhB under visible light (λ > 420 nm) irradiation, 1.2 mol % found to be highly...
Two-dimensional (2D) nanomaterials have been the focus of substantial research interest recently owing to their fascinating and excellent properties. However, 2D porous materials remained quite rare due difficulty creating pores in nanostructures. Here, we synthesized a novel type single-layered mesoporous TiO2 nanosheets with very uniform size thickness as well ordered mesostructure from an unprecedented hydrothermal-induced solvent-confined assembly approach. The F127/TiO2 spherical...
Abstract The rational design of effective catalysts for sluggish oxygen evolution reactions (OERs) is desired but challenging. Nickel‐iron (NiFe) (oxy)hydroxides are promising pre‐electrocatalysts alkaline OER. However, OER performances limited by the slow reconstruction process to generate active species high‐valance NiFe oxyhydroxides. In this work, a sulfate ion (SO 4 2− ) modulated strategy developed boost activity (oxy)hydroxide accelerating electrochemical pre‐catalyst and stabilizing...
The design of Pt-based nanoarchitectures with controllable compositions and morphologies is necessary to enhance their electrocatalytic activity. Herein, we report a rational synthesis anisotropic mesoporous Pt@Pt-skin Pt3Ni core-shell framework nanowires for high-efficient electrocatalysis. catalyst has uniform structure an ultrathin atomic-jagged Pt nanowire core Pt-skin shell, possessing high activity, stability utilisation efficiency. For the oxygen reduction reaction, demonstrated...
Nanostructured carbon materials have received considerable attention due to their special physicochemical properties. Herein, ordered mesoporous carbons (OMCs) with two-dimension (2D) hexagonal mesostructure and unique buckled large mesopores successfully been synthesized via a micelle fusion–aggregation assembly method by using poly(ethylene oxide)-block-polystyrene (PEO-b-PS) diblock copolymers as template resorcinol-based phenolic resin precursor. The obtained possess fiber-like...
The shape of gold: title catalyst has been prepared through a colloidal deposition method. Scanning transmission electron microscopy studies confirmed that for the catalyst, gold clusters with bilayer structure and diameter about 0.5 nm are not mandatory to achieve high activity (see image).
Uniform mesoporous single-crystal TiO 2 spheres with radial channels from driving orientation assembly can be used for energy storage.
High-power sodium-ion batteries (SIBs) with long-term cycling attract increasing attention for large-scale energy storage. However, traditional SIBs toward practical applications still suffer from low rate capability and poor cycle induced by pulverization amorphorization of anodes at high (over 5 C) during the fast ion insertion/extraction process. The present work demonstrates a robust strategy variety (Sb-C, Bi-C, Sn-C, Ge-C, Sb-Bi-C) freestanding metal-carbon framework thin films via...
Constructing three-dimensional (3-D) hierarchical mesostructures with unique morphology, pore orientation, single-crystal nature, and functionality remains a great challenge in materials science. Here, we report confined microemulsion self-assembly approach to synthesize an unprecedented type of 3-D highly ordered mesoporous TiO2 superstructure (Level-1), which consists 1 spherical core 12 symmetric satellite hemispheres epitaxially growing out the vertices. A more complex asymmetric...
Engineering surface structure can precisely and effectively tune the optoelectronic properties of halide perovskites, but are incredibly challenging. Herein, design fabrication uniform all-inorganic CsPbBr3 cubic/tetrahedral single-crystals reported with precise control (100) (111) anisotropy, respectively. By combining theoretical calculations, it is demonstrated that preferred engineering enables a lowest bandgap energy (2.33 eV) high-rate carrier mobility up to 241 μm2 V-1 s-1 ,...
Abstract Porous carbons have been extensively studied in electrochemical capacitors (ECs). However, low capacitance remains a limitation due to the electrical double layer (EDL) storage mechanism when porous are used ionic liquids (ILs) based ECs. Herein, nitrogen‐derived vacancy defects carbon nanospheres found which can boost capacitive charge and present reversible high of 427 F g −1 pure IL electrolyte, equal normalized area (C A ) 16 µF cm −2 , surpassing theoretical EDL C (≈11 ). When...
Titania nanoflakes modified with gold nanoparticles (NPs) were successfully prepared by depositing of Au NPs onto TiO2 using a direct "green" process in the absence organic capping agents. The photocatalyst has been characterized transmission electron microscopy, X-ray photoelectron spectroscopy, diffraction, and UV−vis diffuse reflectance spectroscopy. Results these analyses revealed that (∼1 nm) are homogeneously dispersed on surface highly crystalline (anatase) narrow size distribution....
3D porous hierarchical Cu2S microsponges (HCMs) constructed from 2D ultrathin active nanosheets (∼1.5 nm) with nearly 99% exposed (111) facets are fabricated by a simple hydrothermal route. The as-prepared HCMs possess an improved visible-light-harvesting ability, high surface area, low electron–hole recombination, and excellent photocatalytic activity for phenol degradation under visible light irradiation. As service to our authors readers, this journal provides supporting information...
Oriented self-assembly between inorganic nanocrystals and surfactants is emerging as a route for obtaining new mesocrystalline semiconductors. However, the actual synthesis of mesoporous semiconductor mesocrystals with abundant surface sites extremely difficult, corresponding physical chemical properties arising from such an intrinsic porous nature, which fundamental importance designing high-efficiency nanostructured devices, have been rarely explored poorly understood. Herein, we report...
A general confined coassembly process has been demonstrated to produce discrete uniform mesoporous carbon microspheres with 0.8-1 μm particle size using 3-D-ordered macroporous silica as the template. The obtained (MC-MSs) have and spherical morphology, variable symmetry (hexagonal p6mm or cubic Im3m) of mesostructures, high specific surface areas (500-1100 m(2)/g), large pore volumes (0.6-2.0 cm(3)/g), highly accessible mesopores (7-10.3 nm). can be easily tuned by simply templates...
Spinel structure nickel ferrite (NiFe2O4) doped graphitic carbon nitride (g-C3N4) photocatalyst NiFe2O4/g-C3N4 was synthesized by the coprecipitation route to enhance photocatalytic activity for visible-light driven degradation of methyl orange. The NiFe2O4 doping content is responsible microstructure and samples. Compared with pure g-C3N4, 2-NiFe2O4/g-C3N4 composite 2.0 wt% exhibited excellent superior stability after five runs degrading orange under visible light irradiation. catalytic...
Well ordered, uniform 3D open macro/mesoporous TiO2 hollow microspheres with highly crystalline anatase thin shells have been successfully synthesized by a simple solvent evaporation-driven confined self-assembly method. The show high energy-conversion efficiency (up to 9.5%) and remarkable photocatalytic activity (with photodegradation of 100% for methylene blue in 12 min under UV light irradiation).
A general solvent‐free assembly approach via directly heating amino acid and mesoporous silica mixtures is developed for the synthesis of a family highly nitrogen‐doped carbons. Amino acids have been used as sole precursors templating series ordered During heating, are melted strongly interact with silica, leading to effective loading improved carbon yields (up ≈25 wt%), thus successful structure replication nitrogen‐doping. Unique mechanisms proposed elucidated semi‐quantitatively by using...
The self-assembly of nanoparticles, a process whereby nanocrystal building blocks organize into even more ordered superstructures, is great interest to nanoscience. Here we report the layer-by-layer assembly 2D perovskite nanosheet blocks. Structural analysis reveals that assembled superlattice nanocrystals match with layered Ruddlesden-Popper phase. This proves reversible, as these can be reversibly exfoliated back their via sonication. study demonstrates opportunity further understand and...