Luyi Chen

ORCID: 0000-0002-8801-9907
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About
Contact & Profiles
Research Areas
  • Advancements in Battery Materials
  • Advanced Battery Materials and Technologies
  • Covalent Organic Framework Applications
  • Supercapacitor Materials and Fabrication
  • Metal-Organic Frameworks: Synthesis and Applications
  • Advanced Battery Technologies Research
  • Advanced battery technologies research
  • Dyeing and Modifying Textile Fibers
  • Conducting polymers and applications
  • Advanced Photocatalysis Techniques
  • Analytical chemistry methods development
  • Luminescence and Fluorescent Materials
  • Graphene research and applications
  • Pigment Synthesis and Properties
  • Electrocatalysts for Energy Conversion
  • MXene and MAX Phase Materials
  • Aerogels and thermal insulation
  • Innovative concrete reinforcement materials
  • Molecular Sensors and Ion Detection
  • Magnetism in coordination complexes
  • Extraction and Separation Processes
  • Carbon and Quantum Dots Applications
  • Microplastics and Plastic Pollution
  • Advanced ceramic materials synthesis
  • Nanomaterials for catalytic reactions

South China Normal University
2021-2025

Shenzhen MSU-BIT University
2025

Sun Yat-sen University
2014-2024

Hangzhou Normal University
2022-2024

Donghua University
2014-2023

Ministry of Ecology and Environment
2023

Wuhan Children's Hospital
2021-2023

Huazhong University of Science and Technology
2021-2023

China Railway Major Bridge Reconnaissance & Design Institute (China)
2022

Wuhan Textile University
2021

Abstract Exceptionally large surface area and well-defined nanostructure are both critical in the field of nanoporous carbons for challenging energy environmental issues. The pursuit ultrahigh while maintaining definite remains a formidable challenge because extensive creation pores will undoubtedly give rise to damage nanostructures, especially below 100 nm. Here we report that high up 3,022 m 2 g −1 can be achieved hollow carbon nanospheres with an outer diameter 69 nm by simple...

10.1038/ncomms8221 article EN cc-by Nature Communications 2015-06-15

Lithium-sulfur (Li-S) batteries, based on the redox reaction between elemental sulfur and lithium metal, have attracted great interest because of their inherently high theoretical energy density. However, severe polysulfide shuttle effect sluggish kinetics in cathodes, as well dendrite growth lithium-metal anodes are obstacles for practical application. Herein, a two-in-one approach with superhierarchical cobalt-embedded nitrogen-doped porous carbon nanosheets (Co/N-PCNSs) stable hosts both...

10.1002/adma.201706895 article EN Advanced Materials 2018-02-09

Abstract Aqueous Zn‐metal batteries are the most promising system for large‐scale energy storage due to their high capacity, safety, and low cost. The anode, however, suffers from continuous parasitic reactions, random dendrite growth, sluggish kinetics in aqueous electrolytes. Herein, a donor number solvent, tetramethylurea (TMU), is introduced as electrolyte additive enable highly reversible where TMU can 1) preferentially adsorb on Zn surface inhibit corrosion suppress reaction, 2)...

10.1002/adfm.202209642 article EN Advanced Functional Materials 2022-10-10

Lithium-sulfur (Li-S) batteries has been regarded as one of the most promising next-generation energy storage systems due to their high theoretical density. However, practical application Li-S is still hindered by unstable cathode-electrolyte interphase and early passivation charge product (Li2S), leading poor cycling stability low S utilization. Herein, we propose an electrolyte engineering strategy using highly solvating hexamethylphosphoramide (HMPA) a co-solvent elucidate...

10.1002/anie.202423046 article EN Angewandte Chemie International Edition 2025-01-15

Here, the intrinsic driving mechanisms of autogenous shrinkage for Ultra-High Performance Concrete (UHPC) incorporating porous internal curing (IC) medium are detailly investigated, including characterization and monitoring UHPC hydration kinetics, relative humidity (IRH) temperature (IT) fields. The results show that evolution prepared with pre-wet fine aggregate (PFA) undergoes multiple stages. potential expansion drivers IC at super early hardening period identified as extra liquid volume...

10.1016/j.jobe.2022.104622 article EN cc-by Journal of Building Engineering 2022-05-09

Metal–organic frameworks (MOFs) with high surface area, tunable porous structure, and versatile functionality hold great prospects for manipulating ion transport designing high-performance composite solid electrolytes (CSEs). However, the discontinuous poor mechanical support arising from randomly distributed MOF particles lead to insufficient ionic conductivity inferior strength. Herein, a highly efficient robust MOF-based 3D conducting network was rationally designed by in situ grown...

10.1021/acsmaterialslett.3c00077 article EN ACS Materials Letters 2023-03-13

Transformation of metal-organic framework (MOF) particles into thin films is urgently needed for the persistent development well-applicable devices, and recently emerging functional-integrated hybrid frameworks. Although some flexible polymers exclusive modification approaches have been proposed, additive-free widely applicable strategy has not reported, hampering deep investigation structure-performance relationship. A universal in situ growth large-area continuous MOF with controllable...

10.1002/smll.202307976 article EN Small 2024-03-11

A nitrogen-doped ordered mesoporous carbon/silica nanocomposite with a uniform interface structure was fabricated and demonstrated an impressive lithium ion storage capacity.

10.1039/c4nr06611a article EN Nanoscale 2015-01-01

Multifunctionalization of microporous polymers is highly desirable but remains a significant challenge, considering that the current are generally hydrophobic and nonresponsive to different environmental stimuli difficult be carbonized without damage their well-defined nanomorphology. Herein, we demonstrate facile versatile method fabricate water-dispersible, pH/temperature responsive readily carbonizable hairy polymeric nanospheres based on combination hyper-cross-linking chemistry with...

10.1021/jacs.5b08978 article EN Journal of the American Chemical Society 2015-10-01

Super-hierarchical carbons with a unique carbonaceous hybrid nanotube-interconnected porous network were fabricated by utilizing well-defined carbon nanotube@polystyrene bottlebrushes as building blocks.

10.1039/c6sc03961h article EN cc-by-nc Chemical Science 2016-11-24

A novel strategy is developed to produce an FeS–FeNC-decorated hierarchical porous N,S-co-doped carbon (FeS–FeNC@NSC) electrocatalyst <italic>via</italic> introducing volatile FeCl<sub>3</sub> into a porphyrin polymer framework followed by carbonization.

10.1039/d0cc04749j article EN Chemical Communications 2020-01-01

1,2-Dimethoxyethane (DME) has been considered as the most promising electrolyte solvent for Li-metal batteries (LMBs). However, challenges arise from insufficient Li Coulombic efficiency (CE) and poor anodic stability associated with DME-based electrolytes. Here, we proposed a rational molecular design methodology to tailor solvation stable LMBs, where shortening middle alkyl chain of could reduce chelation ability, while increasing terminal increase steric hindrance, affording...

10.1021/acsami.2c13517 article EN ACS Applied Materials & Interfaces 2022-09-21

Abstract The practical application of lithium-metal batteries is hindered by insufficient lithium Coulombic efficiency and uncontrolled dendrite growth, bringing a challenge concerning how to create robust solid electrolyte interphases (SEIs) that can regulate Li + transport protect reactive lithium-metal. Here, we present the rational construction multi-component jigsaw-like artificial SEI integration fluorine-containing silane polyether-containing silane. fluorine-donating group prevents...

10.1038/s43246-023-00343-w article EN cc-by Communications Materials 2023-02-22

Abstract Diversifying the connecting junctions will be feasible for controllable collaboration of metal–organic frameworks (MOFs) and covalent organic (COFs) to rationally design multifunction‐integrated heterostructures with enhanced performance, yet it is in nascent stage. Herein, by intelligently exploiting polymerization vinyl group, C−C bond innovatively introduced construct core–shell MOF@COF adjustable shell thickness rare interpenetrated structure. The unique structure endows...

10.1002/anie.202412279 article EN Angewandte Chemie International Edition 2024-07-26

Both high surface areas and well‐orchestrated nanomorphologies are important for porous organic polymers (POPs). However, the two key characteristics generally difficult to be satisfied simultaneously, because common pore‐making procedures usually produce ill‐defined or give rise damage of precustomized nanomorphologies. Herein, a facile yet versatile stepwise crosslinking strategy fabrication POPs with an unusual nanomorphology‐persistent characteristic during is reported. Polystyrene...

10.1002/adma.201700723 article EN Advanced Materials 2017-05-08

Nonstoichiometric silica suboxides (SiOx) have been regularly investigated as hopeful anode materials for the substitutions of silicon. However, inherently poor conductivity SiOx limits its promotion in industry. Herein, propose enhanced and stability SiOx-based materials, a kind multicomponent nanosheet (rGO@SiOx@C) is designed fabricated successfully. This progressive design consists inner substrate from reduced graphene oxide (rGO), an intermediate layer SiOx, nitrogen-doped nanoporous...

10.1021/acsaem.0c00084 article EN ACS Applied Energy Materials 2020-03-11
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