- Electrocatalysts for Energy Conversion
- Advanced battery technologies research
- 2D Materials and Applications
- Advancements in Battery Materials
- Supercapacitor Materials and Fabrication
- Graphene research and applications
- Advanced Photocatalysis Techniques
- MXene and MAX Phase Materials
- Advanced Battery Materials and Technologies
- Fuel Cells and Related Materials
- Solar-Powered Water Purification Methods
- Building Energy and Comfort Optimization
- Urban Heat Island Mitigation
- Thermal Radiation and Cooling Technologies
- Perovskite Materials and Applications
- Quantum and electron transport phenomena
- Hybrid Renewable Energy Systems
- Membrane Separation Technologies
- Extraction and Separation Processes
- TiO2 Photocatalysis and Solar Cells
- Hydrogen Storage and Materials
- Advanced Memory and Neural Computing
- Thermodynamic and Exergetic Analyses of Power and Cooling Systems
- CO2 Reduction Techniques and Catalysts
- Energy Harvesting in Wireless Networks
Nanyang Technological University
2019-2024
Abstract The lithium–sulfur (Li–S) battery is widely regarded as a promising energy storage device due to its low price and the high earth‐abundance of materials employed. However, shuttle effect lithium polysulfides (LiPSs) sluggish redox conversion result in inefficient sulfur utilization, power density, rapid electrode deterioration. Herein, these challenges are addressed with two strategies 1) increasing LiPS kinetics through catalysis, 2) alleviating by enhanced trapping adsorption...
Despite the tremendous progress of coupling organic electrooxidation with hydrogen generation in a hybrid electrolysis, electroreforming raw biomass coupled to green has not been reported yet due rigid polymeric structures biomass. Herein, we electrooxidize most abundant natural amino biopolymer chitin acetate over 90% yield electrolysis. The overall energy consumption electrolysis can be reduced by 15% thermodynamically and kinetically more favorable oxidation water oxidation. In obvious...
Abstract The ability to achieve dual‐mode thermal regulation for switchable heating and cooling on a single platform has thus far been challenged by the availability of suitable materials. materials need possess both high solar reflectance transmittance, necessitating large small thicknesses in same coating layer, respectively (i.e., thickness constraint). Herein, first time, single‐layer made facile one‐step process is reported, which exhibits rapid switch between reflection (≈96.6%)...
Abstract Transition metal oxides hold great promise for lithium‐ion batteries (LIBs) and electrocatalytic water splitting because of their high abundance energy density. However, designing fabrication efficient, stable, power density electrode materials are challenging. Herein, we report rambutan‐like hollow carbon spheres formed by nanosheet decorated with nickel oxide (NiO) rich in vacancies (denoted as h ‐NiO/C) a bifunctional material LIBs oxygen evolution reaction (OER). When being used...
Abstract Due to the growing demand for clean and renewable hydrogen fuel, there has been a surge of interest in electrocatalytic water‐splitting devices driven by energy sources. However, feasibility self‐driven water splitting is limited inefficient connections between functional modules, lack highly active stable electrocatalysts, intermittent unpredictable supply. Herein, we construct dual‐modulated three‐dimensional (3D) NiCo 2 O 4 @NiCo S (denoted as NCONCS) heterostructure deposited on...
Abstract MXenes, which are graphene-like two-dimensional transition metal carbides and nitrides, have tunable compositions exhibit rich surface chemistry. This compositional flexibility has resulted in exquisitely electronic, optical, mechanical properties leading to the applications of MXenes catalysis, electronics, energy storage. The work function is an important fundamental property that dictates suitability for these applications. We present a series machine learning models predict...
Abstract Alkaline water electrolysis (AWE) holds great promise for a truly sustainable energy future if it can be driven by renewable sources such as solar and wind. The main challenge arises from the serious partial loading issue when intermittent unstable is coupled to electrolyzers. An storage device mitigate this incompatibility between electrolyzer sources. Herein, an AWE photovoltaic (PV) through full cell of lithium‐ion battery (LIB) reservoir demonstrated (PV−LIB−AWE). Stable power...
Abstract Solar irradiation is a promising resource for sustainable energy conversion and storage in many technological fields. Interfacial solar steam generator emerging as system water harvesting under natural irradiance. However, sunlight usually insufficient conventional interfacial (2D absorber) generators to achieve high efficiency (>85%). Herein, functionalized MXene‐polymeric membrane‐based heat localization structure reported an efficient desalination system. The MXene flakes are...
The creation of pseudo-magnetic fields in strained graphene has emerged as a promising route to allow observing intriguing physical phenomena that would be unattainable with laboratory superconducting magnets. Scanning tunneling spectroscopy experiments have successfully measured the pseudo-Landau levels and proved existence various systems. These giant observed highly deformed can substantially alter optical properties beyond level feasible an external magnetic field, but experimental...
Investigations on external electrostatic field (EEF)-enhanced liquid water evaporation have been reported decades ago, which suggest that molecular alignment and polarization tuned by EEF accelerating the phase change process could be responsible for EEF-enhanced evaporation. However, a detailed study revealing role of in altering intermolecular intramolecular structure is lacking. Herein, an proved to tune state thermal movement molecules, lowering escaping energy, loosening hydrogen bond...
Abstract Arbitrary disposal of plastic waste into landfills and oceans can disturb the ecological system even challenge human survival. Centralized recycling process only works for selected types plastics (e.g., polyethylene) with limited contribution (<10%), because high infrastructure requirement. Comparatively, photoreforming commodity fuels production is much more facile decentralizable, thus holds great potential to mitigate challenge. To this end, a fully solar powered...
Core–shell nanowires with conductive metal cores and active catalyst shells hold great promise for making a electrode high total activity. Indeed, core–shell nanowire arrays have been demonstrated as the in various electrochemical reactions, yet their catalytic roles are underexplored carbon dioxide (CO2) electroreduction. Herein, we report reduced silver@silver chloride (Ag@AgClx) array electrocatalytic CO2 reduction. The Ag@AgClx shows activity including low onset potential current...
Two-dimensional (2D) catalysts often show extraordinary activity at low mass loading since almost all their atoms are exposed to electrolyte. Palladium (Pd) holds great promise for catalyzing oxygen reduction reaction (ORR) but 2D Pd-based ORR catalyst has rarely been reported. Herein, ternary palladium phosphoronitride (Pd3P2Nx) is synthesized, the first time, catalysis. The synthesis guided by a rational design using first-principles density functional theory calculations, and then...
Exciton/trion-involved optoelectronic properties have attracted exponential amount of attention for various applications ranging from optoelectronics, valleytronics to electronics. Herein, we report a new chemical (MXene) doping strategy modulate the negative trion and neutral exciton achieving high photoluminescence yield atomically thin transition metal dichalcogenides, enabled by regulation carrier densities promote electron-bound trion-to-exciton via charge transfer TMDCs MXene. As proof...
<italic>In situ</italic> lithiation-delithiation treatment enables high oxygen reduction activity in palladium selenide without serious structural or phase change; resulting an optimum balance of catalytic and stability.
Abstract In this work, we successfully synthesize a hierarchical porous N‐doped carbon material via low‐cost, facile and scalable spray‐drying method followed with subsequent pyrolysis. This unique delivers excellent electrochemical properties in lithium‐ion batteries (LIBs) sodium‐ion (SIBs) high reversible capacity long cycle life selectivity for CO 2 reduction. The good performance results from the novel structure, which is favor of electrolyte penetration, electron transfer, structural...
The work function of MXenes is crucial in detuning that perovskite materials employed the development optoelectronic devices, to enhance efficiency charge transfer at interfaces.