Bekele Hailegnaw

ORCID: 0000-0003-4427-2772
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About
Contact & Profiles
Research Areas
  • Perovskite Materials and Applications
  • Conducting polymers and applications
  • Chalcogenide Semiconductor Thin Films
  • Quantum Dots Synthesis And Properties
  • Organic Electronics and Photovoltaics
  • Organic Light-Emitting Diodes Research
  • Electrocatalysts for Energy Conversion
  • Advanced battery technologies research
  • Electronic and Structural Properties of Oxides
  • Advanced Sensor and Energy Harvesting Materials
  • Fuel Cells and Related Materials
  • Catalysis for Biomass Conversion
  • Moringa oleifera research and applications
  • Thermal Radiation and Cooling Technologies
  • Biofuel production and bioconversion
  • ZnO doping and properties
  • Carbohydrate Chemistry and Synthesis
  • Optical properties and cooling technologies in crystalline materials
  • Advanced Thermodynamics and Statistical Mechanics
  • Advanced Materials and Mechanics
  • Nanoparticles: synthesis and applications
  • Micro and Nano Robotics
  • Ga2O3 and related materials

Johannes Kepler University of Linz
2018-2025

University of Stuttgart
2025

Weizmann Institute of Science
2015-2016

Bahir Dar University
2015

The great promise of hybrid organic-inorganic lead halide perovskite (HOIP)-based solar cells is being challenged by its Pb content and sensitivity to water. Here, the impact rain on methylammonium iodide films was investigated exposing such water varying pH values, simulating exposure rain. amount loss determined using both gravimetric inductively coupled plasma mass spectrometry measurements. Using our results, extent environment, in case catastrophic module failure, evaluated. Although...

10.1021/acs.jpclett.5b00504 article EN The Journal of Physical Chemistry Letters 2015-04-07

Abstract High-speed locomotion is an essential survival strategy for animals, allowing populating harsh and unpredictable environments. Bio-inspired soft robots equally benefit from versatile ultrafast motion but require appropriate driving mechanisms device designs. Here, we present a class of small-scale electromagnetic made curved elastomeric bilayers, driven by Lorentz forces acting on embedded printed liquid metal channels carrying alternating currents with voltages several volts in...

10.1038/s41467-022-32123-4 article EN cc-by Nature Communications 2022-08-09

The issue of long‐term stability is one the main obstacles challenging progress perovskite solar cells (PSCs). To alleviate this issue, a thorough understanding degradation mechanisms device required. Herein, electrochemical impedance measurements in combination with maximum power point (MPP) tracking are applied to characterize PSCs, aiming gain an charge carrier dynamics photoactive bulk and at contact‐absorber‐interfaces under operation. Electrochemical spectroscopy (EIS) results show...

10.1002/pssa.202000291 article EN cc-by physica status solidi (a) 2020-09-28

Biological synthesis of silver nanoparticles (AgNPs) is a green, simple, cost-effective, time-efficient, and single-step method. This study mainly focused on the using essential oil Laggera tomentosa (LTEO) investigates their potential applications. Ultraviolet-Visible (UV-Vis) result showed characteristic Surface Plasmon Resonance (SPR) peak LTEO-AgNPs at 420 nm. Fourier transform infrared (FT-IR) spectroscopy indicated functional groups present in LTEO LTEO-AgNPs. Scanning electron...

10.3390/su15010797 article EN Sustainability 2023-01-01

All-inorganic perovskites, such as CsPbI2Br, have emerged promising compositions due to their enhanced thermal stability. However, they face significant challenges susceptibility humidity. In this work,...

10.1039/d4ee02385d article EN cc-by Energy & Environmental Science 2025-01-01

X-ray detectors play a pivotal role in development and advancement of humankind, from far-reaching impact medicine to furthering the ability observe distant objects outer space. While other electronics show adapt flexible lightweight formats, state-of-the-art rely on materials requiring bulky fragile configurations, severely limiting their applications. Lead halide perovskites is one most rapidly advancing novel with success field semiconductor devices. Here, an ultraflexible, lightweight,...

10.1002/advs.202002586 article EN Advanced Science 2020-11-13

Abstract Outstanding improvement in power conversion efficiency (PCE) over 25% a very short period and promising research developments to reach the theoretical PCE limit of single junction solar cells, 33%, enables organic–inorganic perovskite cells (OIPSCs) gain much attention scientific industrial community. The simplicity production OIPSCs from precursor solution either on rigid or flexible substrates makes them even more attractive for low-cost roll-to-roll processes. Though show as such...

10.1007/s40243-021-00206-9 article EN cc-by Materials for Renewable and Sustainable Energy 2021-12-27

Incorporating large organic cations to form 2D and mixed 2D/3D structures significantly increases the stability of perovskite solar cells. However, due their low electron mobility, aligning sheets ensure unimpeded charge transport is critical rival high performances pure 3D systems. While additives such as methylammonium chloride (MACl) can enable this preferential orientation, so far, no complete description exists explaining how they influence nucleation process grow highly aligned...

10.1002/adma.202208061 article EN cc-by Advanced Materials 2022-10-28

The development of ambient-air-processable organic–inorganic halide perovskite solar cells (OIHPSCs) is a challenge necessary for the transfer laboratory-scale technology to large-scale and low-cost manufacturing such devices. Different approaches like additives, antisolvents, composition engineering, different deposition techniques have been employed improve morphology films. Additives that can form Lewis acid–base adducts are known minimize extrinsic impacts trigger defects in ambient air....

10.1021/acsomega.3c07592 article EN cc-by-nc-nd ACS Omega 2024-01-04

Nanoscale investigations by scanning probe microscopy have provided major contributions to the rapid development of organic–inorganic halide perovskites (OIHP) as optoelectronic devices. Further improvement device level properties requires a deeper understanding performance-limiting mechanisms such ion migration, phase segregation, and their effects on charge extraction both at nano- macroscale. Here, we studied dynamic electrical response Cs0.05(FA0.83MA0.17)0.95PbI3–xBrx perovskite...

10.1021/acsami.0c10641 article EN cc-by ACS Applied Materials & Interfaces 2020-09-24

Abstract The noticeable growth in the power conversion efficiency of solution-processed organo-inorganic halide perovskite solar cells (OIHPSCs) incited photovoltaic community to look for limitations that hurdle commercialization process. surface and interface defects between electron transport layers are among main challenges cause significant non-radiative recombination losses, thereby they result poor performance stability. In this work, tetracyanoquinodimethane (TCNQ), a strong acceptor...

10.1007/s40243-024-00280-9 article EN cc-by Materials for Renewable and Sustainable Energy 2025-01-21

In this research, cobalt-doped Ni(OH)2 on a PANI-decorated NF substrate is prepared via an electrochemical method. The surface characteristics, roughness, chemical composition, and crystalline structure of the materials are described using scanning electron microscopy (SEM), atomic force (AFM), energy dispersive spectroscopy (EDS), X-ray photoelectron (XPS), diffraction (XRD), in that order. Further, optical characterization techniques attenuated total reflection Fourier transform infrared...

10.1021/acsomega.4c06966 article EN cc-by-nc-nd ACS Omega 2025-02-23

Nowadays, hydrogen fuel is becoming more popular, and it attracting significant attention as a sustainable environmentally benign energy source owing to its zero emission of harmful substances high density. Hydrogen generation through the electrocatalytic evolution reaction (HER) employs economically inexpensive self-supported electrocatalysts that hold immense potential provide cost-effective in future scenario. A NiO@TiO2 nanofiber composite on Ti-foil synthesized via hydrothermal...

10.1021/acs.jpcc.4c00006 article EN The Journal of Physical Chemistry C 2024-03-22

A low temperature solution processed TiO<sub>x</sub>interlayer was used to improve the performance and stability of mixed-cation–mixed-halide perovskite solar cells.

10.1039/c8ra03993c article EN cc-by RSC Advances 2018-01-01

Based on the knowledge that o-aminomethylphenylboronic acids reversibly bind to carbohydrates, relevant water-soluble derivatives of former were prepared by appending hydrophilic tethers. In this way phenylboronic acid used hydrolytically dissolve, i.e. depolymerize cellulose in water at nearly neutral pH values. Some these tethers consisted moieties surmised be able promote hydrolysis glycosidic bonds such as a carboxylic acid, phosphonic weak Bronsted acids, or an imidazole functionality...

10.1021/acssuschemeng.6b01071 article EN publisher-specific-oa ACS Sustainable Chemistry & Engineering 2016-09-06

In this contribution, we show CH3NH3PbI3–xClx perovskite solar cells (PSCs) processed in ambient air from a solution containing the diketone, acetylacetone (AA) solvent as an additive. PSCs with AA additive enhanced photovoltaic properties. The optimized PSC 10 vol % shows average open-circuit voltage (VOC) of about 1.02 V, short-circuit current density (Jsc) around 18.7 mA/cm2, fill factor 76%, and power conversion efficiency 14.5%. Atomic force microscopy topographic imaging depicts that...

10.1021/acs.jpcc.9b05058 article EN The Journal of Physical Chemistry C 2019-09-09

Herein, the optoelectronic properties of interface‐engineered perovskite 2D|3D‐heterojunction structure solar cells are reported. The reciprocity theorem is applied to determine maximum open‐circuit voltage ( V oc ) device can deliver under illumination. A 1.295 found, analyzing measured external quantum efficiency and assuming only radiative recombination. For comparison, experimental found for studied 2D|3D heterojunctions 1.15 V. contribution nonradiative recombination explored by...

10.1002/solr.201900126 article EN cc-by-nc Solar RRL 2019-05-14

The operational stability of organic-inorganic halide perovskite based solar cells is a challenge for widespread commercial adoption. mobility ionic species key contributor to instability since ion migration can lead unfavourable changes in the crystal lattice and ultimately destabilisation phase. Here we study nanoscale early-stage degradation mixed-halide mixed-cation films under operation-like conditions using electrical scanning probe microscopy investigate formation surface nanograin...

10.1039/d1nr05045a article EN cc-by Nanoscale 2022-01-01

Abstract The unprecedented increase in power conversion efficiency (PCE) of low‐cost organo‐inorganic halide perovskite solar cells (OIHPSCs) toward its Shockley‐Queisser limit intriguingly has prompted researchers to investigate the disadvantages these devices. issue operational stability is main hurdle challenging way forward for commercialization. To address this, various engineering processes like composition, additives, anti‐solvents, bulk and interface passivation, deposition...

10.1002/ese3.1745 article EN cc-by Energy Science & Engineering 2024-04-09

Herein, the impact of thin layer polyphosphazene derivatives, as a buffer between electron‐transporting and back metal‐contact in mixed‐cation mixed‐halide perovskite solar cells (PSCs), is explored. PSCs with poly[bis(allylamino)phosphazene] (PPz) interlayer exhibit enhanced rectification photo‐induced current density–voltage ( J–V ) curves, which show improved photovoltaic performance photostability reduced hysteresis. The thickness optimized PPz shows an average open‐circuit voltage V OC...

10.1002/pssa.201900436 article EN physica status solidi (a) 2019-07-04

Photon cooling <italic>via</italic> anti-Stokes photoluminescence (ASPL) is a promising approach to realize all-solid-state cryo-refrigeration by photoexcitation.

10.1039/d0nr04545d article EN cc-by-nc Nanoscale 2020-01-01

Perovskite Solar Cells In article 2208061, Lukas E. Lehner, Martin Kaltenbrunner, and co-workers report the controlled nucleation of quasi-2D perovskites at liquid–air interface precursor solution. Restricting initial crystal growth to surface liquid results in highly aligned perovskite thin films with improved charge transport, enabling efficient solar cells excellent stability.

10.1002/adma.202370030 article EN Advanced Materials 2023-02-01
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