A5086778924- Catalysis for Biomass Conversion
- Catalysis and Hydrodesulfurization Studies
- Catalysts for Methane Reforming
- Coal and Coke Industries Research
- Asymmetric Hydrogenation and Catalysis
- Zeolite Catalysis and Synthesis
- Biofuel production and bioconversion
- Thermochemical Biomass Conversion Processes
- Carbon dioxide utilization in catalysis
- Lignin and Wood Chemistry
- Surface Chemistry and Catalysis
- Electrocatalysts for Energy Conversion
- Quinazolinone synthesis and applications
- Catalysis and Oxidation Reactions
- Hybrid Renewable Energy Systems
- Petroleum Processing and Analysis
- Catalytic Processes in Materials Science
- Chemical Looping and Thermochemical Processes
- CO2 Reduction Techniques and Catalysts
- Phytochemical compounds biological activities
- Multicomponent Synthesis of Heterocycles
- Process Optimization and Integration
- Synthesis and Biological Evaluation
- Oil, Gas, and Environmental Issues
- Covalent Organic Framework Applications
Taiyuan University of Technology
2021-2024
Dalian Institute of Chemical Physics
2016-2023
Chinese Academy of Sciences
2016-2023
Dalian National Laboratory for Clean Energy
2016-2021
University of Chinese Academy of Sciences
2017-2021
Dalian University
2018-2021
Dalian University of Technology
2018-2021
Shanghai Normal University
2019-2021
Kunming University of Science and Technology
2019
University of Jinan
2009
Biomass is renewable and the most abundant carbon resource, it shows great potential for sustainable production of chemicals in future. With respect to limited fossil reserves, biomass conversion has aroused global attention. The use as a resource developed rapidly recent years, various kinds could be produced from biomass. Although annually abundant, important process efficient way. Before rushing into conversion, necessary consider what are reasonably economically In this Review, we first...
To reduce greenhouse gas (GHG) emissions, biomass has been increasingly developed as a renewable and clean alternative to fossil fuels because of its carbon-neutral characteristics. China investigating the rational development use bioenergy for developing energy achieving carbon neutrality. Substituting with multi-source multi-approach utilized corresponding reduction in remain largely unexplored. Here, comprehensive accounting model multi-dimensional analysis was by combining spatial, life...
Biomass reforming by harvesting solar energy can provide green hydrogen. Current biomass photoreforming provides H2 erratically and in limited yield although efficiently, owing to intermittent features of light incomplete degradation C–C bonds. Here, we detour the flaws prioritizing conversion carbohydrates liquid hydrogen carriers (LHCs, consisting HCOOH HCHO), appropriate for transportation. Subsequently, LHCs are fully decomposed, releasing only CO2. This stepwise process enables complete...
Lignin is a renewable and abundant aromatic polymer found in plants. We herein propose "cutting tail" methodology to produce phenol from lignin, which achieved by combining Ru/CeO2 catalyst CuCl2 oxidant via an oxidation–hydrogenation route. Phenol was obtained separated poplar lignin with 13 wt % yield. Even raw biomass, such as poplar, birch, pine, peanut, bamboo willow, straw, could be converted into 1–33 mg per gram of biomass.
Abstract Natural gas is one of the foremost basic energy sources on earth. Although biological process appears as promising valorization routes to transfer biomass sustainable methane, recalcitrance lignocellulosic major limitation for production mixing meet natural composition pipeline transportation. Here we develop a catalytic-drive approach directly solid bio-natural which can be suitable current infrastructure. A catalyst with Ni 2 Al 3 alloy phase enables nearly complete conversion...
Value decomposition (VD) has become one of the most prominent solutions in cooperative multi-agent reinforcement learning. Most existing methods generally explore how to factorize joint value and minimize discrepancies between agent observations characteristics environmental states. However, direct may result limited representation or difficulty optimization. Orthogonal designing a new factorization scheme, this paper, we propose Heterogeneous Policy Fusion (HPF) integrate strengths various...
Hydrogen (H2) has emerged as an ideal, clean, and versatile energy carrier, which would play important role in providing a more competitive economy the future. Owing to recalcitrance structure of biomass with complex composition, achieving high-efficiency H2 production from lignocellulosic under mild conditions remains challenging. Here, catalytic-drive strategy was developed accomplish direct transformation raw relative low-temperature. The nickel–molybdenum catalyst enabled almost complete...
Abstract Quinazolinones, an important class of heterocyclic compounds, have been widely used in pharmaceuticals because their biological activity. However, the efficient and economical synthesis quinazolinones has remained a challenge. A novel synthetic approach now developed to produce from olefins, CO, amines over heterogeneous Ru‐clusters/ceria catalyst absence acids, bases, oxidants. Furthermore, H 2 O is generated as only by‐product. series with aromatic or non‐aromatic substituents can...
Abstract Valuable polyester monomers and plasticizers—1,4‐cyclohexanedimethanol (CHDM), 1,4‐cyclohexanedicarboxylic acid (CHDA), 1,2‐cyclohexanedicarboxylates—have been prepared by a new strategy. The synthetic processes involve proline‐catalyzed formal [3+1+2] cycloaddition of formaldehyde, crotonaldehyde, acrylate (or fumarate). CHDM is produced after subsequent hydrogenation step over commercially available Cu/Zn/Al catalyst one‐pot hydrogenation/oxidation/hydrolysis process yields CHDA,...
Development of an efficient cocatalyst system to eliminate the intrinsic conflict cross-interactions in a pair cocatalysts and overcome extrinsic reaction conditions unmatched environment has great significance asymmetric dual catalysis. Herein, compartmentalization method involving integration been developed, which enables Michael addition/reduction enantioselective dual-catalysis process be accomplished from noncompatible system. In this process, chiral squaramide species is encapsulated...
Abstract Unification of oxidation and reduction in a one‐pot deracemization process has great significance the preparation enantioenriched organic molecules. However, intrinsic mutual deactivation oxidative reductive catalysts extrinsic incompatible reaction conditions are unavoidable challenges single operation. To address these two issues, we develop supported dual system to overcome conflicts from incompatibility compatibility, resulting an efficient redox secondary alcohols. During this...
Abstract Quinazolinones, an important class of heterocyclic compounds, have been widely used in pharmaceuticals because their biological activity. However, the efficient and economical synthesis quinazolinones has remained a challenge. A novel synthetic approach now developed to produce from olefins, CO, amines over heterogeneous Ru‐clusters/ceria catalyst absence acids, bases, oxidants. Furthermore, H 2 O is generated as only by‐product. series with aromatic or non‐aromatic substituents can...