A5101625357- Electrocatalysts for Energy Conversion
- Catalytic Processes in Materials Science
- Advanced Photocatalysis Techniques
- Sleep and related disorders
- Advanced battery technologies research
- X-ray Diffraction in Crystallography
- Crystallization and Solubility Studies
- Electrochemical Analysis and Applications
- Sleep and Wakefulness Research
- Schizophrenia research and treatment
- Catalysis and Oxidation Reactions
- Mental Health Treatment and Access
- Photonic and Optical Devices
- Sleep and Work-Related Fatigue
- Terahertz technology and applications
- Oxidative Organic Chemistry Reactions
- Ammonia Synthesis and Nitrogen Reduction
- CO2 Reduction Techniques and Catalysts
- Obsessive-Compulsive Spectrum Disorders
- Fuel Cells and Related Materials
- Superconducting and THz Device Technology
- Dementia and Cognitive Impairment Research
- Family Caregiving in Mental Illness
- Transcranial Magnetic Stimulation Studies
- MXene and MAX Phase Materials
Guangdong Provincial People's Hospital
2019-2025
Zhejiang University of Technology
2020-2025
Guangdong Academy of Medical Sciences
2017-2025
Southern Medical University
2021-2025
Tianjin University
2012-2024
Huaqiao University
2013-2024
Guangdong Polytechnic of Science and Technology
2024
Zhuhai Institute of Advanced Technology
2023-2024
Shanghai Advanced Research Institute
2016-2023
Chinese Academy of Sciences
2016-2023
Selective cleavage of C–C linkages is the key and a challenge for lignin degradation to harvest value-added aromatic compounds. To this end, electrocatalytic oxidation presents promising technique by virtue mild reaction conditions strong sustainability. However, existing electrocatalysts (traditional bulk metal oxides) bond oxidative suffer from poor selectivity low product yields. We show first time that atomically dispersed Pt–N3C1 sites planted on nitrogen-doped carbon nanotubes...
Abstract Electrooxidation of 5‐hydroxymethylfurfural (HMF) into 2,5‐furandicarboxylic acid (FDCA) is a highly promising approach for producing value‐added chemicals from biomass. However, developing efficient electrocatalysts HMF oxidation (HMFOR) with high current density in large‐scale productions remains challenge. Herein, it demonstrated that the Mn‐doped NiS nanosheet grown directly on 3D graphite felt (GF) substrates can efficiently perform electrooxidation FDCA at industrial‐level...
Abstract The rational design and construction of efficient inexpensive bifunctional oxygen electrocatalysts are highly desirable for the development rechargeable Zn–air batteries (ZABs). Although single‐atom Fe sites anchored on N‐doped carbon catalysts (Fe 1 /NC) ensure high reduction reaction activity, their unitary atomically dispersed active center faces difficult condition in catalyzing evolution simultaneously. Herein, a composite catalyst containing heterointerface between /NC...
Lignin is the most abundant aromatic polymer from natural and renewable lignocellulosic biomass resource. Developing highly efficient catalysts for lignin depolymerization to produce valuable monophenols with high yield selectivity remains a desirable but challenging target in this field. Here, we design synergistic catalyst combining atomically dispersed Mo centers Al Lewis acid sites on MgO substrate (Mo1Al/MgO) of Eucalyptus via β-aryl ether bond cleavage. A near-theoretical monophenol...
Electrochemical alcohol oxidation (EAO) represents an effective method for the production of high-value carbonyl products. However, its industrial viability is hindered by suboptimal efficiency stemming from low reaction rates. Here, we present a synergistic electrocatalysis approach that integrates active electrode and aminoxyl radical to enhance performance EAO. The optimal (4-acetamido-2,2,6,6-tetramethylpiperidine 1-oxyl) Ni0.67V0.33-layered double hydroxide (LDH) are screen as...
Abstract Single‐atom nanozymes (SAzymes), with their superior enzyme‐like catalytic activity, have emerged as promising candidates for oncology therapeutics. The well‐defined structures of SAzymes make them well predictable by experiences and theoretical calculation. However, the effects metal center species coordination environments on activity are variable, screening artificial experiments is challenging. High‐throughput can rapidly select optimal thus better application in tumor therapy...
Assembled from [Th48 Ni6 ] nanocages, the first transition-metal (TM)-thorium metal-organic framework (MOF, 1) has been synthesized and structurally characterized. 1 exhibits high solvent acid/base stability, resistance to 400 kGy β irradiation. Notably, captures ReO4- (an analogue of radioactive 99 TcO4- , a key species in nuclear wastes) with maximum capacity 807 mg g-1 falling among largest values known date. Furthermore, can enrich methylene blue (MB) also serve as an effective...
Environment-friendly electrochemical ozone production (EOP) is a promising route for in situ sterilization and discoloration applications. Herein, Pt-SAs/BNC catalyst with Pt single atoms embedded into B/N codoped nanotubes rationally designed prepared. The process provides local environment rich oxygen intermediates hence improves the EOP performance neutral media by influencing thermodynamics kinetics. exhibits excellent Faraday efficiency of 21% at current density 50 mA cm–2, which almost...
Abstract Clear recognition and rational construction of suitable active center for specific reaction is always great significance in designing highly efficient catalysts. Herein, a dual‐active‐site copper catalyst (DAS‐Cu) containing both CuN 3 4 sites reported. Such catalysts show extremely high catalytic performance (yield: up to 97%) toward oxyphosphorylation alkenes, while with single site (CuN or ) are chemically inert this reaction. Combined theoretical experimental results, the...
Replacing the oxygen evolution reaction (OER) with thermodynamically favorable electrooxidation of organics is considered a promising approach for simultaneous production hydrogen (H2 ) and high-value chemicals. However, exploring optimizing efficient electrocatalysts remains challenge large-scale value-added steroid carbonyl H2 . Herein, Cr-NiO/GF Cr-Ni3 N/GF (GF: graphite felt) were designed as anode cathode carbonyls , respectively. The cooperative Cr-NiO ACT...
Pattern of sleep duration and its correlates have rarely been reported in China. This study examined the relationship with sociodemographic variables, lifestyle, mental health, chronic diseases a large Chinese adult population.This cross-sectional used multistage stratified cluster sampling. A total 17,320 participants from Jilin province were selected interviewed using standardized assessment tools. Basic socio-demographic clinical data collected. Sleep was classified as short (< 7 h per...
Oxidative coupling of methane (OCM) is a catalytic partial oxidation process that converts directly to valuable C2 products (ethane and ethylene). The main difficulties from further investigation this reaction are due the nature its high operating temperature severe exothermicity. In work, an especially designed online characterization setup applied for reaction, which achieved both precise bed control real-time product measurement. High-resolution temperature-dependent rates OCM (CO2,...
This study examined the frequency of mobile phone dependence in Chinese university students and explored its association with social support impulsivity. Altogether, 909 were consecutively recruited from a large China. Mobile use, dependence, impulsivity, measured standardized instruments. The possible use was 78.3% 7.4%, respectively. Multinomial logistic regression analyses revealed that compared no significantly associated being male (p = 0.04, OR 0.7, 95% CI: 0.4-0.98), excessive <...
Efficient formation of valuable multicarbon products in CO2 electrochemical reduction is challenging, owing to the difficulty C-C coupling. Medium micropores embedded channel walls nitrogen-doped ordered mesoporous carbon are found capably promote ethanol production from electroreduction. By scaling up medium micropore content, yield increased 2.3 mmol gcat-1 h-1 , far outperforming previously reported state-of-the-art electrocatalysts. The intrinsically higher activity attributed...
Two-dimensional (2D) materials have been developed into various catalysts with high performance, but employing them for developing highly stable and active nonprecious hydrogen evolution reaction (HER) still encounters many challenges. To this end, the machine learning (ML) screening of HER is accelerated by using genetic programming (GP) symbolic transformers typical 2D MA2Z4 materials. The values Gibbs free energy adsorption (ΔGH*) are accurately rapidly predicted via extreme gradient...
Mental health literacy (MHL) is rarely reported in the Chinese elderly. This study explored pattern of MHL elderly relation to depression, anxiety and poor sleep quality.A cross-sectional was conducted among older adults Guangzhou, south China. Participants were investigated face-to-face using National Health Literacy Scale, Patient Questionnaire-9 item (PHQ-9), 7-item Generalized Anxiety Disorder (GAD-7) Pittsburgh Sleep Quality Index (PSQI). Scale contains three dimensions: mental...