- Advanced Photocatalysis Techniques
- TiO2 Photocatalysis and Solar Cells
- Advanced Nanomaterials in Catalysis
- Arsenic contamination and mitigation
- Supercapacitor Materials and Fabrication
- Electrocatalysts for Energy Conversion
- Catalytic Processes in Materials Science
- Advanced battery technologies research
- Electronic and Structural Properties of Oxides
- Gas Sensing Nanomaterials and Sensors
- Advancements in Battery Materials
- X-ray Diffraction in Crystallography
- Iron oxide chemistry and applications
- Crystallization and Solubility Studies
- Advanced Battery Materials and Technologies
- Copper-based nanomaterials and applications
- Quantum Dots Synthesis And Properties
- Carbon and Quantum Dots Applications
- Ammonia Synthesis and Nitrogen Reduction
- ZnO doping and properties
- Synthesis and Biological Evaluation
- Adsorption and biosorption for pollutant removal
- Nanoplatforms for cancer theranostics
- Gold and Silver Nanoparticles Synthesis and Applications
- Transition Metal Oxide Nanomaterials
Chinese Academy of Sciences
2010-2025
Shenzhen Institutes of Advanced Technology
2022-2025
Hong Kong Polytechnic University
2018-2024
Tianjin Medical University General Hospital
2024
Liaoning University of Technology
2022-2024
University of Illinois Urbana-Champaign
2011-2023
Quzhou University
2023
Zhejiang University
2023
University of Science and Technology of China
2021
Peking University
2005-2017
Even though the well-established Haber-Bosch process has been major artificial way to "fertilize" earth, its energy-intensive nature motivating people learn from nitrogenase, which can fix atmospheric N2 NH3 in vivo under mild conditions with precisely arranged proteins. Here we demonstrate that efficient fixation of proceed room temperature and pressure water using visible light illuminated BiOBr nanosheets oxygen vacancies absence any organic scavengers precious-metal cocatalysts. The...
Incorporating carbon into Bi3O4Cl enhances its internal electric field by 126 times, which induces a bulk charge separation efficiency (ηbulk) of 80%. This ultrahigh ηbulk value presents state-of-the-art result in tuning the separation. The generated C-doped has noble-metal- and electron-scavenger-free water-oxidation ability under visible light, is difficult to achieve with most existing photocatalysts. As service our authors readers, this journal provides supporting information supplied...
Understanding the chemistry of hydrogen peroxide (H2O2) decomposition and hydroxyl radical (•OH) transformation on surface molecular level is a great challenge for application heterogeneous Fenton system in fields chemistry, environmental, life science. We report this study conceptual oxygen vacancy associated without any metal ions leaching, exhibiting unprecedented based electron-donor nature heterolytic H2O2 dissociation. By controlling delicate structure catalyst, novel allows facile...
A central issue in understanding photocatalytic water splitting on a stoichiometric or defective nanostructured oxide surface is its adsorption mode and related reactivity. More than just improving the of surfaces, we demonstrate this work that oxygen vacancies (OVs) also offer possibility activating toward thermodynamically enhanced oxidation, while activation state, as reflected by capability to trap holes, strongly depends structures OVs. Utilizing well-ordered BiOCl single-crystalline...
The distinct structures of oxygen vacancies on different BiOCl facets strongly affect their solar N<sub>2</sub> fixation <italic>via</italic> a proton-assisted electron transfer pathway.
Lightweight and flexible energy storage devices are urgently needed to persistently power wearable devices, lithium-sulfur batteries promising technologies due their low mass densities high theoretical capacities. Here we report a high-energy full battery device with only 100% oversized lithium, enabled by rationally designed copper-coated nickel-coated carbon fabrics as excellent hosts for lithium sulfur, respectively. These metallic endow mechanical flexibility, reduce local current...
A novel Cu2O/TiO2 composite photocatalyst structure of Cu2O nanospheres decorated with TiO2 nanoislands were synthesized by a facile hydrolyzation reaction followed solvent-thermal process. In this photocatalyst, served as the main visible light absorber, while formed heterojunctions good contact Cu2O, beneficial to photoexcited electron transfer between them. Their band match and inner electrostatic field from p–n heterojunction both favored electrons TiO2, which effectively separated...
Electrochemical ammonia (NH3) synthesis from nitrate (NO3-) reduction offers an intriguing approach for both sustainable and environmental denitrification, yet it remains hindered by a complicated reaction pathway with various intermediates. Here we present that the interlayer strain compression in bismuth (Bi) nanocrystals can contribute to activity selectivity improvement toward NH3 electrosynthesis NO3- reduction. By virtue of comprehensive spectroscopic studies theoretical calculations,...
Prussian blue analogs (PBAs) are promising catalysts for green hydrogen production. However, the rational design of high-performing PBAs is challenging, which requires an in-depth understanding catalytic mechanism. Here FeMn@CoNi core-shell employed as precursors, together with Se powders, in low-temperature pyrolysis argon atmosphere. This synthesis method enables partial dissociation inner FeMn that results hollow interiors, Ni nanoparticles (NPs) exsolution to surface, and incorporation...
The creation of photocatalysts with controlled facets has become an important approach to enhance their activity. However, how the formation heterojunctions on exposed could affect photocatalytic performance ranking had not yet been investigated. In this study, Cu2O@TiO2 core–shell structures were created, and Cu2O/TiO2 p–n formed various Cu2O cubes, cuboctahedra, octahedra, respectively. These polyhedra demonstrated enhanced degradation effect Methylene Blue (MB) 4-nitrophenol (4-NP) under...
A visible light photocatalyst is synthesized by dispersing palladium oxide nanoparticles on nitrogen-doped n-titanium oxide. The demonstrates not only a much faster photocatalytic disinfection rate Escherichia coli under illumination than titanium oxide, but also "memory" catalytic capability. These unusual antimicrobial properties of TiON/PdO are derived from strong optoelectronic coupling between PdO and TiON semiconductor.
Surface reactions of 2,5-diethynyl-1,4-bis(phenylethynyl)benzene on Ag(111), Ag(110), and Ag(100) were systematically explored scrutinized by scanning tunneling microscopy, molecular mechanics simulations, density functional theory calculations. On Glaser coupling reaction became dominant, yielding one-dimensional wires formed covalent bonds. Ag(110) Ag(100), however, the terminal alkynes reacted with surface metal atoms, leading to organometallic nanostructures. Detailed experimental...
A type of highly efficient completely flexible fiber-shaped solar cell based on TiO2 nanotube array is successfully prepared. Under air mass 1.5G (100 mW cm−2) illumination conditions, the photoelectric conversion efficiency approaches 7%, highest among all cells arrays and first DSSC. The demonstrates good flexibility, which makes it suitable for modularization using weaving technologies.
Abstract Because of the large abundance sodium (Na) as a source material and easy fabrication Na‐containing compounds, battery is more environmentally friendly sustainable technology than lithium‐ion (LIB). Na‐metal batteries (SMBs) are considered promising to realize high energy density overtake cost effectiveness LIBs, which critically important in large‐scale applications such grid storage. However, cycling stability anode faces significant challenges particularly under capacities, due...