Paolo Rosi

ORCID: 0000-0002-5789-6763
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Research Areas
  • Advanced Electron Microscopy Techniques and Applications
  • Orbital Angular Momentum in Optics
  • Near-Field Optical Microscopy
  • Electron and X-Ray Spectroscopy Techniques
  • Random lasers and scattering media
  • Digital Holography and Microscopy
  • Electrohydrodynamics and Fluid Dynamics
  • Optical Polarization and Ellipsometry
  • Spectroscopy Techniques in Biomedical and Chemical Research
  • Spectroscopy and Chemometric Analyses
  • Magnetic properties of thin films
  • Advanced Fluorescence Microscopy Techniques
  • Electrowetting and Microfluidic Technologies
  • Characterization and Applications of Magnetic Nanoparticles
  • Photosynthetic Processes and Mechanisms
  • Advanced X-ray Imaging Techniques
  • Optical measurement and interference techniques
  • Engineering Applied Research
  • Engineering Structural Analysis Methods
  • Cell Image Analysis Techniques
  • Advanced Optical Imaging Technologies
  • Data Analysis with R
  • Spreadsheets and End-User Computing
  • Gyrotron and Vacuum Electronics Research
  • Statistical and Computational Modeling

University of Modena and Reggio Emilia
2020-2025

Istituto Nanoscienze
2018-2024

We report the first experimental demonstration of an electrostatic electron orbital angular momentum (OAM) sorter, which can be used to analyze OAM states electrons in a transmission microscope. verify sorter functionality for several beams possessing different superpositions states, and use it record spectra. Our current has resolution 2 units h/bar - reduced Planck constant. It is expected increase optimal 1 future via fine control sorting phase elements.

10.1103/physrevlett.126.094802 article EN cc-by Physical Review Letters 2021-03-05

The experimentally retrieved value of the optical extinction cross section per unit length, σL,extNT, individual MoS2 multiwall nanotubes (NTs) is here reported over 440–940 nm wavelength range for light polarization both parallel and perpendicular to nanotube longitudinal axis. impact diameter environment on σL,extNT addressed with diameters 120 220 in suspended, sapphire-supported, PMMA-supported configurations. Measuring utmost importance given wide size dispersion intrinsic synthesis...

10.1021/acs.jpcc.4c08613 article EN The Journal of Physical Chemistry C 2025-02-27

We report the use of an electrostatic micro-electromechanical systems-based device to produce high quality electron vortex beams with more than 1000 quanta orbital angular momentum (OAM). Diffraction and off-axis holography experiments are used show that diameter in diffraction plane increases linearly OAM, thereby allowing content be calibrated. The realization even larger values OAM is currently limited by breakdown voltage device. Potential solutions overcome this problem discussed.

10.1063/5.0093411 article EN Applied Physics Letters 2022-08-15

With operando transmission electron microscopy visualizing the solid–solid electrode–electrolyte interface of silicon active particles and lithium oxide solid electrolyte as a model system, we show that (de)lithiation (battery cycling) does not require all to be in direct contact with electrolytes across length scales few hundred nanometers. A facile redistribution occurs between interconnected indicates necessarily become isolated individual due loss contact. Our results have implications...

10.1021/acsaem.0c00543 article EN cc-by-nc-nd ACS Applied Energy Materials 2020-05-08

A convolutional neural network is used to align an orbital angular momentum sorter in a transmission electron microscope. The method demonstrated using simulations and experiments. As result of its accuracy speed, it offers the possibility real-time tuning other optical devices beam shaping configurations.

10.1016/j.ultramic.2021.113338 article EN cc-by-nc-nd Ultramicroscopy 2021-06-18

Solving challenges of enhanced imaging (resolution or speed) is a continuously changing frontier research. Within this sphere, ghost (and the closely related single-pixel imaging) has evolved as an alternative to focal plane detector arrays owing advances in detectors and/or modulation devices. The interest these techniques due their robustness varied sets patterns and applicability broad range wavelengths compatibility with compressive sensing. To achieve better control illumination...

10.34133/icomputing.0001 article EN Intelligent Computing 2022-01-01

Beam shaping - the ability to engineer phase and amplitude of massive massless particles has long interested scientists working on communication, imaging foundations quantum mechanics. In light optics, electromagnetic waves (photons) can be achieved using techniques that include, but are not limited to, direct manipulation beam source (as in X-ray Free Electron Lasers (XFELs) Synchrotrons), deformable mirrors, spatial modulators, mode converters holograms. The recent introduction holographic...

10.1063/5.0067528 article EN cc-by Journal of Applied Physics 2022-01-18

Chirality can appear at many length scales in nature. In this study the authors introduce planar chirality as a quantitative geometric measure of for two-dimensional objects. They apply to evaluate nanometer-sized structures with an electron microscope. employ innovative electron-optics device, orbital-angular-momentum sorter, which applies log-polar conformal mapping wave function and reaches near-optimal resolution orbital angular momentum.

10.1103/physrevapplied.22.014083 article EN Physical Review Applied 2024-07-31

By means of numerical simulations, we demonstrate the innovative use computational ghost imaging in transmission electron microscopy to retrieve images with a resolution that overcomes limitations imposed by coherent aberrations. The method requires measuring intensity on single pixel detector series structured illuminations. success technique is improved if probes are made resemble sample and patterns cover area interest evenly. using simple 8 electrode device as specific example, twofold...

10.1103/physrevlett.133.123801 article EN cc-by Physical Review Letters 2024-09-18

Abstract We report on the automatic alignment of a transmission electron microscope equipped with an orbital angular momentum sorter using convolutional neural network. The network is able to control all relevant parameters both electron-optical setup and external voltage source without input from user. It can compensate for mechanical optical misalignments sorter, in order optimize its spectral resolution. completed over few frames be kept stable by making use fast fitting time

10.1017/s143192762201248x article EN Microscopy and Microanalysis 2022-09-11

By means of numerical simulations, we demonstrate the innovative use computational ghost imaging in transmission electron microscopy to retrieve images with a resolution that overcomes limitations imposed by coherent aberrations. The method requires measuring intensity on single pixel detector series structured illuminations. success technique is improved if probes are made resemble sample and patterns cover area interest evenly. using simple 8 electrode device as specific example, 2-fold...

10.48550/arxiv.2401.01898 preprint EN cc-by arXiv (Cornell University) 2024-01-01

<title>Abstract</title> Rotational invariance is a fundamental aspect of symmetry in scattering processes from atomic potentials. Here, we introduce new approach for measuring orbital angular momentum (OAM), key descriptor rotational symmetry, during measurements transitions. We use an electron optical ‘OAM sorter’ combination with energy-loss spectroscopy (EELS) to perform unified spectral analysis the π* and σ* anti-bonding transitions hexagonal boron nitride on scale. The allows...

10.21203/rs.3.rs-4606043/v1 preprint EN Research Square (Research Square) 2024-07-05

Abstract Tuneable phase plates for free electrons are a highly active area of research. However, their widespread implementation, similar to that spatial light modulators in optics, has been hindered by both conceptual and technical challenges. A specific challenge involves the need minimize obstruction electron beam supporting films electrodes. Here, we describe numerical analytical mathematical frameworks three-dimensional stacks can be used provide near-arbitrary shaping with minimal obstruction.

10.1093/mam/ozae108 article EN cc-by Microscopy and Microanalysis 2024-11-26

The orbital angular momentum (OAM) sorter is an electron optical device for the measurement of electron's OAM. It based on two phase elements, which are referred to as "unwrapper" and a "corrector" located in Fourier conjugate planes. simplest implementation electrostatic such charged needle unwrapper electrodes with alternating charges or potentials corrector. Here, we use formal analogy between shifts introduced by vertical currents propose alternative designs magnetic fields. We this...

10.1016/j.ultramic.2021.113287 article EN cc-by-nc-nd Ultramicroscopy 2021-04-21

Modern nanotechnology techniques offer new opportunities for fabricating structures and devices at the micrometer sub-micrometer level. Here, we use focused ion beam to realize micrometer-sized Janus bimetallic cylinders acting as drift tube devices, which are able impart a controlled phase shift an electron wave. The results from presence of contact potentials in cylinders, similar manner electrostatic Aharonov–Bohm effect wires. We Fraunhofer interference demonstrate that such introduce...

10.1063/5.0050055 article EN Journal of Applied Physics 2021-07-12

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10.1017/s143192762100324x article EN Microscopy and Microanalysis 2021-07-30

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10.1017/s1431927620019212 article EN Microscopy and Microanalysis 2020-07-30

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10.1017/s1431927620018449 article EN Microscopy and Microanalysis 2020-07-30

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10.1017/s1431927622008637 article EN Microscopy and Microanalysis 2022-07-22

We report on the automatic alignment of a transmission electron microscope equipped with an orbital angular momentum sorter using convolutional neural network. The network is able to control all relevant parameters both electron-optical setup and external voltage source without input from user. It compensate for mechanical optical misalignments sorter, in order optimize its spectral resolution. completed over few frames can be kept stable by making use fast fitting time

10.48550/arxiv.2111.05032 preprint EN cc-by arXiv (Cornell University) 2021-01-01
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