- Luminescence and Fluorescent Materials
- Organic Light-Emitting Diodes Research
- Nanoplatforms for cancer theranostics
- Molecular Sensors and Ion Detection
- Photoreceptor and optogenetics research
- Photodynamic Therapy Research Studies
- Advanced Sensor and Energy Harvesting Materials
- Perovskite Materials and Applications
- Polydiacetylene-based materials and applications
- Conducting polymers and applications
- Organic Electronics and Photovoltaics
- Luminescence Properties of Advanced Materials
- X-ray Diffraction in Crystallography
- Quantum Dots Synthesis And Properties
- Nicotinic Acetylcholine Receptors Study
- Synthesis and properties of polymers
- Analytical Chemistry and Sensors
- Advanced biosensing and bioanalysis techniques
- Solar-Powered Water Purification Methods
- Membrane Separation Technologies
- Crystallization and Solubility Studies
- Photochromic and Fluorescence Chemistry
- Solar Thermal and Photovoltaic Systems
- Advanced Nanomaterials in Catalysis
Sun Yat-sen University
2021-2025
Shenzhen University
2020
Materials Science & Engineering
2020
Organic near infrared (NIR) persistent-luminescence systems with bright and long-lived emission are highly valuable for applications in communication, imaging, sensors. However, realizing these materials (especially lifetime over 0.1 s) is a challenge, mainly because of non-radiative quenching their excitons. Herein, universal strategy stepwise Förster resonance energy transfer (FRET) NIR system remarkable persistent luminescence (up to 0.2 s at 810 nm) presented, based on new...
Abstract Organic type‐I photosensitizers (PSs) which produce aggressive reactive oxygen species (ROS) with less oxygen‐dependent exhibit attractive curative effect for photodynamic therapy (PDT), as they adapt better to hypoxia microenvironment in tumors. However, the reported PSs are limited and its exacted mechanism of dependence is still unclear. Herein, new selenium‐containing Se6 Se5 benzoselenadiazole acceptor has been designed possessed aggregation‐induced emission characteristic....
Developing stable room-temperature phosphorescence (RTP) emission without being affected by moisture and mechanical force remains a great challenge for purely organic systems, due to their triplet states sensitive the infinitesimal motion of phosphors oxygen quencher. We report kind highly robust phosphorescent doping rigid phosphor into copolymer (polyvinyl butyral resin) matrix with balance mutually exclusive features, including rigidly hydrophilic hydrogen bond network elastically...
Perovskite light-emitting diodes (PeLEDs) emerge as a promising class of optoelectronic devices for next-generation displays and lighting technology. However, the performance blue PeLEDs lags far behind that their green red counterparts, including unachieved trade-off between high efficiency luminance, severe roll-off, unsatisfactory power efficiency. Here, multi-functional chiral ligand L-phenylalanine methyl ester hydrochloride is strategically introduced into quasi-2D perovskites, which...
It remains challenging to develop organic afterglow materials with a variable emission color and not single during decay. Herein, we developed kind of time-dependent multicolor polyurethane (PU) system whose can undergo four distinct changes within 1.0 s. The rapid UV-cured copolymerization pyrene-1-carboxylate derivative (PyC) poly(ε-caprolactone) (PCL) prepolymer ensured that the resulting PU systems possessed dual persistent luminescence phosphorescence at 626 nm lifetime over 200 ms...
A kind of NIR afterglow with a lifetime 0.16 s at 808 nm was prepared using triplet excimer (PVB@PVA) as the donor. PYB 2 @PVA containing more excimers is beneficial to improve luminescence Cy7 acceptor via triplet-to-singlet energy transfer.
The overexpressed glutathione (GSH) in tumor cells was a crucial obstacle to improving the performance of photodynamic therapy (PDT). Complex approaches combined with different substances for PDT and GSH depletion brought potential toxic/side effects metal ions or used unsustainable disulfide bonds. Therefore, photosensitizer (PS) capable continuously depleting keeping reactive oxygen species (ROS) generation from falling simultaneously is still challenge. Here, newly designed Janus-PSs TBBr...
Abstract Mechanically responsive materials (MRMs) usually showing observable changes in emission intensity (mechanochromic) under force stimuli have garnered increasing interest due to their broad range of potential applications. Relative usual mechanochromic materials, a kind alternative MRMs with changeable lifetime upon terms mechanodecay is proposed. A catalog novel both and characteristics reported. Halogen‐free semicrystalline polymers doped chromophores bright ultralong...
The Förster resonance energy transfer (FRET) process has been utilized to construct host–guest systems with stimuli-responsive room-temperature phosphorescence (RTP).
Organic room-temperature phosphorescence (RTP) materials have demonstrated great potential applications in optoelectronics, anticounterfeiting, and biomedicine fields. Among them, the RTP properties of host–guest systems can be easily regulated by changing their component parameters, which has attracted widespread attention. However, key factor hosts (crystalline or noncovalent interaction network) for boosting emission at room temperature was still unclear. Herein, a triphenyl phosphor...
Recent advancements have focused on developing nanoscale persistent room-temperature phosphorescence (pRTP) structures to expand their applicability in biomedical fields. Traditional fabrication methods typically produce surface-coated core-shell pRTP nanoparticles composed of nonbiocompatible emitters at very high concentrations the core. To overcome this limitation, polymeric nanosystems been presented study as a promising alternative by embedding RTP molecules within biocompatible polymer...
Abstract Though mechano‐responsive luminescent materials obtained much attention, most of their responses are non‐reversible, let alone in situ reversible. Here, the study presents a new strategy to push through this limitation for applications, which relies on reversible (MR) hydrogen bonding interactions and polymer chain orientation among doped polyurethane (PU) elastomer. The radiative nonradiative transitions inside these phosphorescent triphenylene‐based aromatic secondary amines (TpNP...
A series of novel AIEgens based on Katritzky pyridinium salts were readily synthesized and exhibited interesting aggregation-induced emission behaviors, remarkable mechanochromic luminescence, promising heparin detection.
Reversible tricolored mechanochromism and recyclable mechanoluminescence properties (new shoots) of a reported tetraphenylethene derivative (old roots) were explored.
AIE active photosensitizer of OMEPYH with benzophenone core and methylpyridinium group exhibited highly efficient generation both type-I type-II reactive oxygen species, which can be used for mitochondria-targeted photodynamic therapy (PDT).
Blue light-emitting materials with excellent film-forming ability, superior morphological stability, outstanding color purity, and high device efficiency are in urgent demand for new-generation display solid-state lighting devices fabricated by low-cost wet processing. However, their current performances far from satisfactory. Herein, two polyimide (PI)-base blue polymers first precisely constructed synthesized through a“Hinge-type Linking”strategy. A small molecular is introduced into the...
Organic non-conjugated materials with room temperature phosphorescence (RTP) have attracted increasing attention due to their fundamental importance and advantages like environmental friendliness, good biocompatibility, various processing methods. However, most systems often suffered from the problem very short RTP lifetimes in ambient conditions. Here, we proposed an efficient strategy improve performance of chitosan (CTS) by constructing a strong ionic bond network based on carboxylic...