Wen Zhao

ORCID: 0000-0002-1118-8155
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About
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Research Areas
  • Advancements in Battery Materials
  • Advanced Battery Materials and Technologies
  • 2D Materials and Applications
  • Advanced battery technologies research
  • MXene and MAX Phase Materials
  • Graphene research and applications
  • Electrocatalysts for Energy Conversion
  • Advanced Photocatalysis Techniques
  • Catalytic Processes in Materials Science
  • Boron and Carbon Nanomaterials Research
  • Supercapacitor Materials and Fabrication
  • Advanced Battery Technologies Research
  • Metal-Organic Frameworks: Synthesis and Applications
  • Topological Materials and Phenomena
  • Advanced Thermoelectric Materials and Devices
  • Nanomaterials for catalytic reactions
  • Ammonia Synthesis and Nitrogen Reduction
  • Adsorption and biosorption for pollutant removal
  • CO2 Reduction Techniques and Catalysts
  • Chemical Synthesis and Characterization
  • Diamond and Carbon-based Materials Research
  • Phosphorus and nutrient management
  • Catalysis and Hydrodesulfurization Studies
  • Quantum Dots Synthesis And Properties
  • Metal and Thin Film Mechanics

China University of Petroleum, East China
2020-2025

State Key Laboratory of Pollution Control and Resource Reuse
2024-2025

Nanjing University
2024-2025

City University of Hong Kong
2024

University of Connecticut
2021-2024

Wuhan University of Technology
2023

Qingdao University of Science and Technology
2022

Institute for Basic Science
2017-2021

Ministry of Education of the People's Republic of China
2021

Northwest University
2021

Nitrogen-doped graphene (NG) is a promising conductive matrix material for fabricating high-performance Li/S batteries. Here we report simple, low-cost, and scalable method to prepare an additive-free nanocomposite cathode in which sulfur nanoparticles are wrapped inside the NG sheets (S@NG). We show that Li/S@NG can deliver high specific discharge capacities at rates, is, ∼1167 mAh g–1 0.2 C, ∼1058 0.5 ∼971 1 ∼802 2 ∼606 5 C. The cells also demonstrate ultralong cycle life exceeding 2000...

10.1021/nl5020475 article EN Nano Letters 2014-07-29

An <italic>in situ</italic> constructed VO<sub>2</sub>–VN binary host was realized to accomplish smooth immobilization–diffusion–conversion of polysulfides, targeting high-sulfur-load Li–S batteries.

10.1039/c8ee01402g article EN Energy & Environmental Science 2018-01-01

Liquid- phase exfoliation (LPE) is the principal method of producing two-dimensional (2D) materials such as graphene in large quantities with a good balance between quality and cost now widely adopted by both academic industrial sectors. The fragmentation mechanisms involved have usually been simply attributed to force induced ultrasound interaction solvent molecules. Nonetheless, little known about how they actually occur, i.e., thick graphite crystals can be exfoliated into thin small...

10.1021/acsnano.0c03916 article EN ACS Nano 2020-06-29

Abstract Lithium–sulfur (Li–S) batteries are deemed to be one of the most promising energy storage technologies because their high density, low cost, and environmental benignancy. However, existing drawbacks including shuttling intermediate polysulfides, insulating nature sulfur, considerable volume change sulfur cathode would otherwise result in capacity fading unstable cycling. To overcome these challenges, herein an situ assembly route is presented fabricate VS 2 /reduced graphene oxide...

10.1002/aenm.201800201 article EN Advanced Energy Materials 2018-04-19

Electrocatalysts remain vitally important for the rational management of intermediate polysulfides (LiPSs) in realm Li-S batteries. In terms transition-metal-based candidates, situ evolution electrocatalysts course an electrochemical process has been acknowledged; nevertheless, consensus not yet reached on their real functional states as well catalytic mechanisms. Herein, we report all-chemical vapor deposition design defective vanadium diselenide (VSe2)-vertical graphene (VG)...

10.1021/acsnano.0c05030 article EN ACS Nano 2020-08-12

Potassium ion batteries (KIB) have become a compelling energy-storage system owing to their cost effectiveness and the high abundance of potassium in comparison with lithium. However, its practical applications been thwarted by series challenges, including marked volume expansion sluggish reaction kinetics caused large radius ions. In line this, exploration reliable anode materials affording electrical conductivity, sufficient active sites, structural robustness is key. The synthesis...

10.1002/smll.201906566 article EN Small 2020-01-23

Ru/RuO 2 composites with unique metal/metal oxide interface are proposed and work to pursue efficient HER performance in pH-universal media.

10.1039/d1ee02380b article EN Energy & Environmental Science 2021-01-01

Metal complexes have shown impressive selectivity and activity as catalysts for electrochemical CO2 reduction (CO2RR), yet the nature of their active sites under operating conditions remains elusive. Herein, by using in situ Raman, X-ray photoelectron spectroscopy, advanced electron microscopy combination with density functional theory calculations, we reveal that copper phthalocyanine (CuPc) reconstructs during CO2RR, which proceeds through demetalation CuPc to Cu atoms followed...

10.1021/acscatal.3c01439 article EN ACS Catalysis 2023-06-28

An in situ electrochemical scanning electronic microscopy method is developed to systematically study the lithium plating/stripping processes liquid electrolytes. The results demonstrate that dendrite growth speed and mechanism greatly affected by additives ether-based electrolyte. As a service our authors readers, this journal provides supporting information supplied authors. Such materials are peer reviewed may be re-organized for online delivery, but not copy-edited or typeset. Technical...

10.1002/adma.201606187 article EN Advanced Materials 2017-01-27

A few-layered Ti<sub>3</sub>C<sub>2</sub>nanosheet/glass fiber composite separator was designed and fabricated as a lithium polysulphide reservoir for high-performance lithium–sulfur batteries.

10.1039/c5ta10307j article EN Journal of Materials Chemistry A 2016-01-01

Exerting synthetic control over the edge structure and chemistry of two-dimensional (2D) materials is critical importance to direct magnetic, optical, electrical, catalytic properties for specific applications. Here, we directly image evolution pores in Mo

10.1038/s41467-018-04435-x article EN cc-by Nature Communications 2018-05-20

The lithium-sulfur (Li-S) battery has been deemed as one of the most promising energy-storage systems owing to its high energy density, low cost, and environmental benignancy. However, capacity decay kinetic sluggishness stemming from polysulfide shuttle effects have by far posed a great challenge practical performance. We herein demonstrate employment low-cost, wet-chemistry-derived VO2 nanobelts effective host additives for graphene-based sulfur cathode. displayed an ultrafast anchoring...

10.1021/acsami.8b02920 article EN ACS Applied Materials & Interfaces 2018-04-24

Abstract Graphdiyne (GDY), an emerging type of carbon allotropes, possesses fascinating electrical, chemical, and mechanical properties to readily spark energy applications in the realm Li‐ion Na‐ion batteries. Nevertheless, rational design GDY architectures targeting advanced K‐ion storage has rarely been reported date. Herein, first example synthesizing frameworks a scalable fashion realize superb potassium for high‐performance battery (KIB) anodes is showcased. To begin with, principles...

10.1002/adfm.202003039 article EN Advanced Functional Materials 2020-06-09

Employing an Al foil current collector at the potassium anode side is ideal choice to entail low-cost and high-energy potassium-metal batteries (PMBs). Nevertheless, poor affinity between planar can cause uneven K plating/stripping and, hence, undermined performance, which remains a significant challenge be addressed. Herein, nitrogen-doped carbon@graphdiyne (NC@GDY)-modified affording potassiophilic properties proposed, simultaneously suppresses dendrite growth prolongs lifespan of anodes....

10.1002/adma.202202685 article EN Advanced Materials 2022-05-20

Phase change materials (PCMs) are increasingly capturing the spotlight in realm of building design and construction owing to their capacity absorb release thermal energy throughout phase transitions. This review provides a comprehensive overview PCMs, outlining properties applications improving efficiency, comfort, sustainability buildings. It delves into various types discussing selection criteria, integration methods, impact on indoor climate consumption. The exploration covers both...

10.1016/j.greenca.2024.03.003 article EN cc-by-nc-nd Green Carbon 2024-03-30

Phase transitions between semiconducting 2H and metallic 1T (or 1T′) molybdenum disulphides (MoS2) are explored comprehensively by first-principles calculations. The nucleation of a nucleus in MoS2 lattice, the formation 2H–1T (1T′) interfaces kinetics interface propagation during phase transition were thoroughly investigated this study. It was found that, among various potential structures two phases, Mo-rich S-rich zigzag (ZZ) boundaries energetically more preferable than others....

10.1039/c6nr08628d article EN Nanoscale 2017-01-01

The high mechanical strength and excellent flexibility of 2D materials such as graphene are some their most important properties [1]. Good is key for exploiting in many emerging technologies, wearable electronics, bioelectronics, protective coatings composites [1] recently bending has been suggested a route to tune electronic transport behaviour [2]. For virtually all crystalline macroscopic deformation accommodated by the movement dislocations through formation twinning defects [3]; it...

10.1038/s41467-018-06074-8 article EN cc-by Nature Communications 2018-08-30

Abstract Sodium (Na) metal batteries are nowadays appealing due to high specific capacity and low cost. However, major caveats including severe Na dendrite growth, unstable solid electrolyte interphase formation, poor mechanical robustness have hampered its practicability. In this report, a highly sodiophilic conductive host harnessing hierarchical vertical graphene (VG) cultivator Co nanoparticle/ N ‐doped carbon decorator (Co‐VG/CC) is designed accommodate throughout facile infusion route....

10.1002/adfm.202101233 article EN Advanced Functional Materials 2021-03-09
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