Shiyan Li

ORCID: 0000-0002-1146-0104
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About
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Research Areas
  • Catalytic Processes in Materials Science
  • Catalysts for Methane Reforming
  • Geophysical Methods and Applications
  • Advancements in Semiconductor Devices and Circuit Design
  • Electrocatalysts for Energy Conversion
  • Catalysis and Hydrodesulfurization Studies
  • Semiconductor materials and devices
  • Geophysical and Geoelectrical Methods
  • Nanomaterials for catalytic reactions
  • Social Robot Interaction and HRI
  • Crystallization and Solubility Studies
  • Industrial Gas Emission Control
  • Nanowire Synthesis and Applications
  • Catalysis and Oxidation Reactions
  • Underwater Acoustics Research
  • Photonic and Optical Devices
  • Seismic Imaging and Inversion Techniques
  • Advanced biosensing and bioanalysis techniques
  • Polymer composites and self-healing
  • Ferroelectric and Negative Capacitance Devices
  • Advanced Photocatalysis Techniques
  • Machine Fault Diagnosis Techniques
  • Marine and coastal plant biology
  • Carbon Dioxide Capture Technologies
  • CRISPR and Genetic Engineering

University of Chinese Academy of Sciences
2021-2025

Dalian National Laboratory for Clean Energy
2019-2025

Dalian Institute of Chemical Physics
2019-2025

Chinese Academy of Sciences
2015-2025

Tianjin Special Equipment Supervision and Inspection Technology Research Institute
2024-2025

Shanghai Institute of Nutrition and Health
2024

Aerospace Information Research Institute
2021-2023

State Key Laboratory of Polymer Physics and Chemistry
2023

Changchun Institute of Applied Chemistry
2023

Xiangtan University
2022

Developing highly efficient catalyst for selective oxidation of benzene to phenol (SOBP) with low H2O2 consumption is desirable practical application, but challenge remains. Herein, we report unique single-atom Cu1-N1O2 coordination-structure on N/C material (Cu-N1O2 SA/CN), prepared by water molecule-mediated pre-assembly-pyrolysis method, can efficiently boost SOBP reaction at a 2:1 H2O2/benzene molar ratio, showing 83.7% high conversion 98.1% selectivity. The sites provide preponderant...

10.1038/s41467-022-34852-y article EN cc-by Nature Communications 2022-11-16

The rational design of high-temperature endurable Cu-based catalysts is a long-sought goal since they are suffering from significant sintering. Establishing barrier on the metal surface by classical strong metal-support interaction (SMSI) supposed to be an efficient way for immobilizing nanoparticles. However, Cu particles were regarded as impossible form SMSI before irreversible Herein, we fabricate between sputtering reconstructed and flame-made LaTiO2 support at mild reduction...

10.1038/s41467-021-27557-1 article EN cc-by Nature Communications 2021-12-10

Directly growing hierarchical nanosheet-based microplate phosphide arrays on Ni foam via a hydrothermal phosphorization process creates an active and durable bifunctional electrocatalyst for overall water splitting in both acidic alkaline media.

10.1039/d1ta04713b article EN Journal of Materials Chemistry A 2021-01-01

Cubic α-phase molybdenum carbides (α-MoC1-x) exhibit great potential in hydrogen production at low temperatures due to their excellent activity water dissociation. However, the design strategies of α-MoC1-x are severely restricted by harsh synthesis conditions, which involve multistep ammonification and carburization or utilization a significant amount noble metals. Herein, high-purity one-step process was achieved with assistance trace Rh (0.02%). The structural evolution Mo species during...

10.1021/jacs.2c08979 article EN Journal of the American Chemical Society 2022-11-23

Selective oxidation of H2S to sulfur is an efficient process for industrial applications and environmental requirement reduce the residual in Claus technology ultralow content (<0.1 ppm) before releasing off-gas into atmosphere. Recently, numerous research studies have been devoted development highly active, selective stable catalysts such fields application. However, there usually a trade-off between conversion selectivity S due inevitable overoxidation or SO2 on active catalysts. In this...

10.1021/acscatal.1c01252 article EN ACS Catalysis 2021-06-30

Abstract Adenine base editors (ABEs) and cytosine (CBEs) enable the single nucleotide editing of targeted DNA sites avoiding generation double strand breaks, however, genomic features that influence outcomes in vivo still remain to be characterized. High-throughput datasets from lentiviral integrated libraries were used investigate sequence affecting outcomes, but effects endogenous factors beyond sequences are largely unknown. Here ABE CBE evaluated mammalian cells for 5012 11,868...

10.1038/s41421-023-00624-1 article EN cc-by Cell Discovery 2024-02-20

Acetaldehyde, the major ethanol metabolite that is far more toxic and reactive than ethanol, has been postulated to be responsible for alcohol-induced tissue cell injury. This study was examine whether facilitated acetaldehyde metabolism affects acetaldehyde-induced oxidative stress apoptosis. Transgene-encoding human aldehyde dehydrogenase-2 (ALDH2), which converts into acetate, constructed under chicken beta-actin promoter transfected umbilical vein endothelial cells (HUVECs). Efficacy of...

10.1074/jbc.m308011200 article EN cc-by Journal of Biological Chemistry 2004-03-01

The post-Claus selective catalytic oxidation of H2S reaction in a continuous mode is demonstrated on N-doped 3D mesoporous carbon/carbon nanotube (N-C/CNT) monoliths at temperature higher than the dew point (>180 °C) elemental sulfur. N-C/CNT display hierarchical open porous framework (an interconnected macroporous–mesoporous network) with abundant active nitrogen species surface and controlled macroscopic size shape which represent prerequisites for operating gas-phase reactions. Physical...

10.1021/acsanm.9b00654 article EN ACS Applied Nano Materials 2019-05-15

The optimization of MgO-based adsorbents as advanced CO2 -capture materials is predominantly focused on their molten-salt modification, for which theoretical and experimental contributions provide great insights high performance. underlying mechanism the promotion effect molten salt capture, however, a topic controversy. Herein, characterization techniques, including in situ environmental transmission electron microscopy (eTEM) chemisorption by diffuse-reflectance infrared Fourier transform...

10.1002/adma.202106677 article EN Advanced Materials 2021-11-03

Multi-interfacial engineering NiS-Ni 2 P/Ni hybrid on Ni foam creates an active and durable electrocatalyst for hydrogen evolution in alkaline or neutral media, also providing a general method preparing other multi-interfacial electrocatalysts.

10.1039/d2ta03021g article EN Journal of Materials Chemistry A 2022-01-01

The high-temperature reverse water–gas shift (RWGS) is an industrially relevant reaction. Cu-based catalysts easily sinter and deactivate under these conditions. We demonstrate that it possible to obtain high-performance stable by modifying the mechanism of action. Cu/CeOx-MgO (denoted as Cu/CexMgy) were developed in which Cu nanoparticles mostly generate spillover H migrates support sites where CO2 selectively reduced, with rate controlled oxide–oxide CeOx-MgO interface. An optimal...

10.1021/acscatal.4c07729 article EN ACS Catalysis 2025-02-12

Recent advancements in geophysical exploration have highlighted the importance of integrating electromagnetic (EM) and magnetic data to enhance subsurface target detection. Conventional inversion techniques often struggle with non-uniqueness solutions sensitivity noise when relying on a single modality. In this study, we introduce novel deep learning framework, MagEMNet, designed jointly invert EM responses. This convolutional neural network (CNN)-based model effectively combines these two...

10.3390/app15063125 article EN cc-by Applied Sciences 2025-03-13

Atom-by-atom control of a catalyst surface is central yet challenging topic in heterogeneous catalysis, which enables precisely confined adsorption and oriented approach reactant molecules. Here, exposed surfaces with either consecutive Pd trimers (Pd3) or isolated atoms (Pd1) are architected for Pd2Ga intermetallic nanoparticles (NPs) using reactive metal-support interaction (RMSI). At elevated temperatures under hydrogen, situ atomic-scale transmission electron microscopy directly...

10.1126/sciadv.abq5751 article EN cc-by-nc Science Advances 2022-12-09

(2020). Relationship between social robot proactive behavior and the human perception of anthropomorphic attributes. Advanced Robotics: Vol. 34, Special Issue on Robot Human Interactive Communication 2020, pp. 1324-1336.

10.1080/01691864.2020.1831699 article EN Advanced Robotics 2020-10-12

The time-domain electromagnetic (TDEM) method is acknowledged for its simplicity in setup and non-intrusive detection capabilities, particularly within shallow subsurface methodologies. However, extant TDEM systems encounter constraints when detecting intricate topographies hazardous zones. rapid evolution unmanned aerial vehicle (UAV) technology has engendered the inception of UAV-based systems, thereby augmenting efficiency while mitigating potential risks associated with human casualties....

10.3390/rs16020330 article EN cc-by Remote Sensing 2024-01-13
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