A5102915603- Electrocatalysts for Energy Conversion
- Ammonia Synthesis and Nitrogen Reduction
- Nanomaterials for catalytic reactions
- Electrochemical Analysis and Applications
- Advanced Photocatalysis Techniques
- Advanced battery technologies research
- Gold and Silver Nanoparticles Synthesis and Applications
- Advanced Nanomaterials in Catalysis
- CO2 Reduction Techniques and Catalysts
- Trigeminal Neuralgia and Treatments
- Botulinum Toxin and Related Neurological Disorders
- Hydrogen Storage and Materials
- Catalytic Processes in Materials Science
- Nanoplatforms for cancer theranostics
- Advanced biosensing and bioanalysis techniques
- Migraine and Headache Studies
- Metal-Organic Frameworks: Synthesis and Applications
- Electrochemical sensors and biosensors
- Caching and Content Delivery
- Machine Learning in Materials Science
- Graphene and Nanomaterials Applications
- Inflammasome and immune disorders
- Pain Mechanisms and Treatments
- Quantum Dots Synthesis And Properties
- Copper-based nanomaterials and applications
University of Science and Technology Beijing
2021-2025
Loudi Central Hospital
2025
East China University of Science and Technology
2021-2024
Wenzhou University
2019-2021
First Affiliated Hospital of Zhengzhou University
2014-2015
Zhengzhou University
2014
Electrocatalytic nitrate (NO3-) reduction to ammonia (NRA) has emerged as an alternative strategy for effluent treatment and production. Despite significant advancements that have been achieved in this field, the efficient conversion of low-concentration at low overpotential remains a formidable challenge. This challenge stems from sluggish reaction kinetics caused by limited distribution negatively charged NO3- vicinity working electrode competing side reactions. Here, pulsed potential...
Abstract As the best electrocatalysts for alcohol oxidation reactions in direct fuel cells (DAFCs), Pt‐based nanomaterials still face challenges of low utilization efficiency Pt atoms and poor reaction kinetics. To address these issues, a self‐etching strategy is developed to prepare PtBi nanorings (NRs) with abundant low‐coordinated inhomogeneous tensile strain (≈4%). The obtained NRs exhibit superior activity toward methanol (MOR) ethanol (EOR) alkaline media. Particularly, mass activities...
Electrocatalytic nitrate (NO
Abstract Background In the majority of cases, trigeminal neuralgia (TN) is a unilateral condition with ultra-short stabbing pain located along one or more branches nerve. Although prophylactic pharmacological treatment first choise, considering insufficient effect unacceptable side effects, neurosurgical lesion should be considered. addition to all these procedures mentioned above, approach has been based on local intradermal and/or submucosal injections Botulinum Toxin Type A (BTX-A)....
ATP and reactive oxygen species (ROS) are considered significant indicators of cell apoptosis. However, visualizing the interplay between apoptosis-related ROS is challenging. Herein, we developed a metal–organic framework (MOF)-based nanoprobe for an apoptosis assay using duplex imaging cellular ROS. The was fabricated through controlled encapsulation gold nanorods with thin zirconium-based MOF layer, followed by modification ROS-responsive molecules 2-mercaptohydroquinone...
Heterophase nanomaterials have sparked significant research interest in catalysis due to their distinctive properties arising from synergistic effects of different components and the formed phase boundary. However, challenges persist controlled synthesis heterophase intermetallic compounds (IMCs), primarily lattice mismatch distinct crystal phases difficulty achieving precise control transitions. Herein, orthorhombic/cubic Ru2Ge3/RuGe IMCs with engineered boundary architecture are...
Constructing amorphous/intermetallic (A/IMC) heterophase structures by breaking the highly ordered IMC phase with disordered amorphous is an effective way to improve electrocatalytic performance of noble metal-based electrocatalysts because optimized electronic structure and abundant boundaries as active sites. In this study, we report synthesis ultrathin A/IMC PtPbBi nanosheets (NSs) for boosting hydrogen evolution reaction (HER) alcohol oxidation reactions. The resulting NSs exhibit a...
Abstract Benefiting from ordered atomic structures and strong d‐orbital interactions, intermetallic compounds (IMCs) are promising electrocatalysts for hydrogen evolution reaction (HER) oxygen (OER). Herein, the body‐centered cubic IrGa IMCs with donor–acceptor architectures synthesized anchored on nitrogen‐doped reduced graphene oxide (i.e., IrGa/N‐rGO). Structural characterizations theoretical calculations reveal that electron‐rich Ir sites atomically dispersed in IrGa/N‐rGO, facilitating...
Atomically ordered Ir 3 Ti intermetallics on carbon nanotubes exhibit remarkable performance for pH-universal overall water splitting.
Abstract Background We investigated the long-term effects and safety of botulinum toxin-A (BTX-A) for treating trigeminal neuralgia (TN). also studied maintenance this therapeutic effect. Methods A visual analog scale (VAS) score, pain attack frequency per day, patient’s overall response to treatment side during 14-month follow-up were evaluated in 88 patients with TN receiving BTX-A. The primary endpoints severity (assessed by VAS) day. secondary endpoint was treatment, assessed using...
Hydrogen peroxide (H2O2) widely involves in intracellular and intercellular redox signaling pathways, playing a vital role regulating various physiological events. Nevertheless, current analytical methods for the H2O2 assay are often hindered by relatively long response time, low sensitivity, or self-interference. Herein, zeolitic imidazolate framework-8 (ZIF-8)-based surface-enhanced Raman scattering (SERS) sensor has been developed to detect released from living cells depositing ZIF-8 over...
Abstract Iridium (Ir) is an efficient catalyst for overall water splitting, yet its widespread utilization hampered by the substantial cost and limited stability. Alloying Ir with heteroatoms can optimize electronic structure of reduce required amount Ir. Compared to solid solution alloys, Ir‐based intermetallic compounds (IMCs) ordered stronger Ir‐heteroatom bonds exhibit superior catalytic activity durability. Hence, adjusting crystal IMCs expected further configurations active sites...
Heart failure (HF) causes structural and functional changes in the heart, with pyroptosis-mediated inflammatory response as core link HF pathogenesis. E3 ubiquitin ligases participate cardiovascular disease progression. Here, we explored underlying molecular mechanisms of ligase Smurf1 governing HF.
Abstract The upcycling of polyethylene terephthalate (PET)‐derived ethylene glycol (EG) to glycolic acid (GA, a biodegradable polymer monomer) via electrocatalysis not only produces valuable chemicals but also mitigates plastic pollution. However, the current reports for electrooxidation EG‐to‐GA usually operate at reaction potentials >1.0 V vs reversible hydrogen electrode (RHE), much higher than theoretical potential (0.065 RHE), resulting in substantial energy wastage. Herein,...
The aims of this study were to investigate the clinical effects and safety botulinum toxin A (BTX-A) in treating trigeminal neuralgia its influences on accompanied depression, anxiety, sleep disorders, quality life.Eighty-seven patients with one-branch classical injected BTX-A pain area. visual analogic scale score, interference Hamilton Anxiety Scale Depression side assessed at 1 week prior 8 weeks after treatment, respectively.The effective rates 1, 2, 4, treatment 48.28%, 66.67%, 78.16%,...
Abstract Metastable‐phase intermetallic compounds (IMCs) provide great flexibility to modify the electronic structure and surface coordination environment of metallic catalysts for various reactions. However, synthesis metastable‐phase IMCs with high catalytic performance remains a challenge due their thermodynamically unstable nature. Here, wet‐chemical epitaxial growth strategy synthesize Pd‐Bi nanocrystals (NCs) is reported. β‐Pd 3 Bi γ‐Pd 5 NCs are epitaxially grown on templates...
Abstract Constructing amorphous/intermetallic (A/IMC) heterophase structures by breaking the highly ordered IMC phase with disordered amorphous is an effective way to improve electrocatalytic performance of noble metal‐based electrocatalysts because optimized electronic structure and abundant boundaries as active sites. In this study, we report synthesis ultrathin A/IMC PtPbBi nanosheets (NSs) for boosting hydrogen evolution reaction (HER) alcohol oxidation reactions. The resulting NSs...
Abstract Gallium (Ga) with a low melting point can serve as unique metallic solvent in the synthesis of intermetallic compounds (IMCs). The negative formation enthalpy transition metal‐Ga IMCs endows them high catalytic stability. Meanwhile, their tunable crystal structures offer possibility to tailor configurations active sites meet requirements for specific applications. Herein, we present general method preparing range IMCs, including Co−Ga, Ni−Ga, Pt−Ga, Pd−Ga, and Rh−Ga IMCs....
Abstract Gallium (Ga) with a low melting point can serve as unique metallic solvent in the synthesis of intermetallic compounds (IMCs). The negative formation enthalpy transition metal‐Ga IMCs endows them high catalytic stability. Meanwhile, their tunable crystal structures offer possibility to tailor configurations active sites meet requirements for specific applications. Herein, we present general method preparing range IMCs, including Co−Ga, Ni−Ga, Pt−Ga, Pd−Ga, and Rh−Ga IMCs....