- Electrochemical sensors and biosensors
- Advanced biosensing and bioanalysis techniques
- Electrochemical Analysis and Applications
- Advanced Nanomaterials in Catalysis
- Analytical Chemistry and Sensors
- X-ray Diffraction in Crystallography
- Ionic liquids properties and applications
- CO2 Reduction Techniques and Catalysts
- Metal-Organic Frameworks: Synthesis and Applications
- Crystallization and Solubility Studies
- Conducting polymers and applications
- Biosensors and Analytical Detection
- Nanocluster Synthesis and Applications
- Advanced Biosensing Techniques and Applications
- Neuroscience and Neural Engineering
- Advanced battery technologies research
- Advanced Sensor and Energy Harvesting Materials
- Magnetism in coordination complexes
- Luminescence and Fluorescent Materials
- Advanced Memory and Neural Computing
- Synthesis and Reactivity of Heterocycles
- Molecular Junctions and Nanostructures
- Advancements in Battery Materials
- Adsorption and Cooling Systems
- Nanoplatforms for cancer theranostics
Capital Normal University
2020-2024
Hefei National Center for Physical Sciences at Nanoscale
2024
University of Science and Technology of China
2024
China University of Petroleum, East China
2023
Nanjing Tech University
2022
Peking University
2016-2021
Beijing National Laboratory for Molecular Sciences
2016-2021
Electrochemiluminescence (ECL) is a highly successful technique used in commercial immunoassays for clinical diagnosis. Developing an ECL-based multiplex immunoassay, with the potential to enable high-throughput detection of multiple biomarkers simultaneously, remains current research interest yet limited by narrow choice ECL luminophores. Herein we report synthesis, photophysics, electrochemistry, and several new ruthenium(II) iridium(III) complexes, three which are eventually as signal...
The lithium-sulfur (Li-S) battery is one of the most promising next generation energy storage systems due to its high theoretical specific energy. However, shuttle effect soluble lithium polysulfides formed during cell operation a crucial reason for low cyclability suffered by current Li-S batteries. As result, an in-depth mechanistic understanding sulfur cathode redox reactions urgently required further advancement Herein, direct observation in reported situ hyphenated technique...
In many electrochemiluminescent (ECL) systems, coreactants play crucial roles in the redox-induced light emission process at electrode surface. this work, a novel and environment-friendly nanoplatform for ECL immunosensing enabled by triethanolamine (TEOA)-modified gold nanoparticles (TEOA@AuNPs) is reported. The monodisperse TEOA@AuNPs are fabricated one-pot synthesis using TEOA as both reducing stabilizing agent. Then TEOA@AuNPs-modified not only acted coreactant Ru(bpy)32+ system but also...
Adenosine triphosphate (ATP) is the major resource of energy supply in tumor activity. Therefore, improving ATP consumption efficiencies a promising approach for cancer therapy. Herein, inspired by H2O2-involved structure regulation effect during catalysis natural protein enzymes, we developed an artificial H2O2-driven catalysis-promoting system, Ce-based metal-organic framework (Ce-MOF), catalytic In presence H2O2, hydrolysis activity Ce-MOF(H2O2) was enhanced around 1.6 times. Taking...
Proton-coupled electron transfer (PCET) reactions at various interfaces (liquid/membrane, solid/electrolyte, liquid/liquid) lie the heart of many processes in biology and chemistry. Mechanistic study can provide profound understanding PCET rational design new systems. However, most mechanisms a liquid/liquid interface have been proposed based on electrochemical spectroscopic data, which lack direct evidence for possible intermediates. Moreover, as one type soft is dynamic, making...
In this work, fullerenols were found to be able enhance the ECL signals of luminol and H2O2 system employed for first time as a reducing, catalyzing, stabilizing agent in one-step fast synthesis fullerenols@AuNPs only 5 min. First, prepared applied fabricate label-free immunosensor detection human cardiopathy biomarker (cardiac troponin I, cTnI). Second, using biolabels establish sandwich-type catalyzing situ copper-stained reaction generate Cu particles capped on fullerenols@AuNPs, then...
Diabetes is a metabolic syndrome associated with hyperglycemia, hypertension, atherosclerosis, and endothelial dysfunction. Applying the mechanical stretch on cells to simulate blood circulation while monitoring cell glucose metabolism in high-glucose environment important for better comprehension of underlying mechanisms atherosclerosis caused by diabetes. Herein, we developed facile strategy integrating zeolitic imidazolate framework-8-encapsulated oxidase (GOx@ZIF-8) an gold (Au)...
Trans-interfacial behaviors of multiple ionic species at the interface between two immiscible electrolyte solutions (ITIES) are importance to biomembrane mimicking, chemical and biosensing, interfacial molecular catalysis. Utilizing host–guest interaction facilitate ion transfer is an effective commonly used method decrease Gibbs energy a target molecule. Herein, we investigated facilitated (FIT) process poly(amidoamine)dendrimer (PAMAM, G0–G2) by dibenzo-18-crown-6 (DB18C6) microinterfaces...
Abstract Electron‐transfer (ET) reactions at a liquid/liquid (L/L) interface have attracted much attention because they are relevant to many important chemical and biological processes. At an L/L interface, the ET reaction is usually coupled with ion‐transfer (IT) reaction, it difficult discriminate between them. Despite great progress that has been made, nature of coupling still unclear two proposed mechanisms subject debate over past several decades. Herein, ferrocene (Fc) in...
{PMo 12 } based rare earth phosphine oxide complexes have good adsorption properties for rhodamine B and can degrade methylene blue under UV irradiation.
Chloride ion, a pivotal cerebral anion involved in neuronal inhibition, is implicated various neurodegenerative diseases. Conventional direct faradaic detection based on electron transfers at solid electrode/solution interfaces has been proven ineffective due to the electrochemically inactive nature of Cl − . Here, we present an approach involving molecularly tailored liquid/liquid interfacial ultramicro iontronics (L/L-UIs) supported ultramicropipettes filled with organic gel containing...
Two new complexes, [Cu(dmp)(2-bdppmapy)](CF3SO3)·CH2Cl2 (1) and [Cu(imidazo[4,5-f])(2-bdppmapy)](SCN) (2) (2-bdppmapy = N,N-bis[(diphenylphosphino)methyl]-2-pyridinamine, dmp 2,9-dimethyl-(1,10)phenanthroline imidazo[4,5-f] 1H-imidazo[4,5f][1,10]phenanthroline), have been synthesized in mixed solvents of CH3OH CH2Cl2 (1:1, V/V). On the basis studying structure photophysical properties Cu(I) effects different N ligands counter anions on luminescence complexes were characterized by...
Compared with typical two-dimensional electrodes, the three-dimensional (3D) cell culture platform can simulate real survival environment for growth to accurately reproduce functions. Moreover, considering that living cells are exposed various of mechanical force in microenvironment, construction 3D electrodes excellent flexible, stretchable, and biocompatibility is great significance real-time monitor mechanically evoked biomolecule release from cells. Herein, we demonstrated a...