Kun Qi

ORCID: 0000-0002-5574-4475
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About
Contact & Profiles
Research Areas
  • Electrocatalysts for Energy Conversion
  • Advanced Photocatalysis Techniques
  • Geological formations and processes
  • CO2 Reduction Techniques and Catalysts
  • Geological and Geophysical Studies
  • Geology and Paleoclimatology Research
  • Copper-based nanomaterials and applications
  • Catalytic Processes in Materials Science
  • Nanomaterials for catalytic reactions
  • Advanced battery technologies research
  • Hydrocarbon exploration and reservoir analysis
  • Ionic liquids properties and applications
  • Scientific Measurement and Uncertainty Evaluation
  • Ammonia Synthesis and Nitrogen Reduction
  • 2D Materials and Applications
  • Advanced biosensing and bioanalysis techniques
  • Electrochemical Analysis and Applications
  • Advanced Frequency and Time Standards
  • earthquake and tectonic studies
  • Membrane Separation Technologies
  • Quantum Dots Synthesis And Properties
  • MXene and MAX Phase Materials
  • Advanced Thermoelectric Materials and Devices
  • Covalent Organic Framework Applications
  • ZnO doping and properties

Beijing Information Science & Technology University
2024-2025

Dalian Institute of Chemical Physics
2024-2025

Chinese Academy of Sciences
2024-2025

Université de Montpellier
2020-2024

École Nationale Supérieure de Chimie de Montpellier
2020-2024

Southwest Petroleum University
2018-2024

State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation
2018-2024

Institut Européen des Membranes
2020-2024

Centre National de la Recherche Scientifique
2020-2024

Dalian National Laboratory for Clean Energy
2024

MicroRNA exhibits differential expression levels in cancer and can affect cellular transformation, carcinogenesis metastasis. Although fluorescence techniques using dye molecule labels have been studied, label-free molecular-level quantification of miRNA is extremely challenging. We developed a surface plasmon resonance sensor based on two-dimensional nanomaterial antimonene for the specific detection clinically relevant biomarkers such as miRNA-21 miRNA-155. First-principles energetic...

10.1038/s41467-018-07947-8 article EN cc-by Nature Communications 2018-12-28

Abstract The grand challenge in the development of atomically dispersed metallic catalysts is their low metal-atom loading density, uncontrollable localization and ambiguous interactions with supports, posing difficulty maximizing catalytic performance. Here, we achieve an interface catalyst consisting atomic cobalt array covalently bound to distorted 1T MoS 2 nanosheets (SA Co-D ). phase transforming from 2H D-1T, induced by strain lattice mismatch formation Co-S covalent bond between Co...

10.1038/s41467-019-12997-7 article EN cc-by Nature Communications 2019-11-19

The precise construction of photocatalysts with diatomic sites that simultaneously foster light absorption and catalytic activity is a formidable challenge, as both processes follow distinct pathways. Herein, an electrostatically driven self-assembly approach used, where phenanthroline used to synthesize bifunctional LaNi within covalent organic framework. La Ni site acts optically catalytically active center for photocarriers generation highly selective CO2-to-CO reduction, respectively....

10.1038/s41467-023-37545-2 article EN cc-by Nature Communications 2023-04-29

Abstract Electrochemical synthesis of NH 3 is a carbon‐free alternative to the traditional Haber–Bosch process. Obtaining from environmental pollutants, such as nitrates or nitrites, more practical route than nitrogen reduction reaction (NRR) due difficult cleavage inert triple bond gas. Here, novel heterogeneous catalyst reported based on iron (Fe) single‐atoms supported 2D MoS 2 (Fe‐MoS ) for nitrate (NO RR). Fe‐MoS exhibits remarkable performance with maximum Faradaic efficiency 98% NO RR...

10.1002/adfm.202108316 article EN Advanced Functional Materials 2021-12-22

Abstract Non-noble metal nanoparticles are becoming more and important in catalysis recently. Cu/CuO nanoclusters on highly ordered TiO 2 nanotube arrays successfully developed by a surfactant-free photoreduction method. This non-noble Cu/CuO-TiO catalyst exhibits excellent catalytic activity stability for the reduction of 4-nitrophenol (4-NP) to 4-aminophenol (4-AP) with presence sodium borohydride (NaBH 4 ). The rate constant this low-cost based is even higher than that noble decorated...

10.1038/srep39695 article EN cc-by Scientific Reports 2017-01-10

Abstract The single-atom nanozyme is a new concept and has tremendous prospects to become next-generation nanozyme. However, few studies have been carried out elucidate the intrinsic mechanisms for both single atoms supports in nanozymes. Herein, heterogeneous Co–MoS 2 (SA ) demonstrated excellent potential as high-performance peroxidase mimic. Because of well-defined structure SA , its peroxidase-like mechanism extensively interpreted through experimental theoretical studies. Due different...

10.1007/s40820-019-0324-7 article EN cc-by Nano-Micro Letters 2019-11-22

A molybdenum disulfide/palladium nanodisk heterostructure was determined to be highly active toward the HER through DFT predictions and experimental verification.

10.1039/c5ta10337a article EN Journal of Materials Chemistry A 2016-01-01

Exploring the nonlinear photonics of emerging promising two-dimensional (2D) materials like MXenes will boost development broad-band optoelectronic and photonic applications. In this paper, optical response excited-carrier dynamics an MXene, Nb2C, are systematically investigated for wavelength range visible to near-infrared band. The obtained shows a excitation intensity dependence. imaginary part third-order susceptibility Imχ(3) figure merit were found be -1.4 × 10-10 esu 7.5 10-12 cm,...

10.1021/acsnano.0c04390 article EN ACS Nano 2020-07-20

Developing cheap, stable, and efficient electrocatalysts is of extreme importance in the effort to replace noble metal for use hydrogen evolution reaction (HER) oxygen (OER). We report a three-dimensional self-supported Cu3P nanobush (NB) catalyst directly grown on copper mesh via one-step method. This nanostructure exhibits superior catalytic activity achieving current density 10 mA cm-2 at 120 mV long-term stability acid solutions. It shows Tafel slope 72 dec-1 an onset potential -44 mV....

10.1021/acsomega.6b00366 article EN publisher-specific-oa ACS Omega 2016-12-22

Tailoring the interfacial structure of Pt-based catalysts has emerged as an effective strategy to improve catalytic activity. However, little attention been focused on investigating relationship between facets and their Here, we design implement Pd-Pt interfaces with controlled heterostructure features by epitaxially growing Pt nanoparticles Pd nanosheets. On basis both density functional theory calculation experimental results, demonstrate that charge transfer from is highly dependent...

10.1021/acsami.7b05290 article EN ACS Applied Materials & Interfaces 2017-05-10

Metallic 1T-phase transition metal dichalcogenides (TMDs) are of considerable interest in enhancing catalytic applications due to their abundant active sites and good conductivity. However, the unstable nature TMDs greatly impedes practical applications. Herein, we developed a new approach for synthesis highly stable Au/Pd-MoS2 nanosheets (NSs) through assembly induced ultrastable phase achieving very high electrocatalytic activity hydrogen evolution reaction. The was evoked by novel...

10.1021/acs.nanolett.8b04104 article EN Nano Letters 2019-04-08

The conversion of CO2 into desirable multicarbon products via the electrochemical reduction reaction holds promise to achieve a circular carbon economy. Here, we report strategy in which modify surface bimetallic silver-copper catalyst with aromatic heterocycles such as thiadiazole and triazole derivatives increase hydrocarbon molecules. By combining operando Raman X-ray absorption spectroscopy electrocatalytic measurements analysis products, identified that electron withdrawing nature...

10.1038/s41467-021-27456-5 article EN cc-by Nature Communications 2021-12-10

Developing active and bifunctional noble metal-free electrocatalysts is crucial for both the oxygen evolution reaction (OER) hydrogen (HER) in full water splitting process. A ternary nanoporous sulfur-doped copper oxide (Cu2OxS1-x) was successfully synthesized on Cu foam. The obtained Cu2OxS1-x/Cu shows robust electrocatalytic activity toward HER with a low overpotential of 40 mV at 10 mA cm-2 Tafel slope 68 dec-1 exhibits long-term stability acid solution. Moreover, Cu2OxS1-x excellent OER,...

10.1021/acsami.7b16280 article EN ACS Applied Materials & Interfaces 2017-12-21

Rational control of the components noble metal alloys is paramount for achieving satisfactory electrocatalytic performances. Though transition metals are commonly used to modify metals, many potential elements remain be explored. Here, we interstitially modulate hydrogen atoms into RhPd nanoparticles boost alkaline evolution reaction (HER). The obtained stable RhPd-H exhibit pronounced HER activity with a small overpotential 36.6 mV at 10 mA cm-2 and low Tafel slope 35.3 dec-1. surface...

10.1021/acsnano.9b05615 article EN ACS Nano 2019-10-16

Abstract Moiré superlattices (MSLs) are modulated structures produced from homogeneous or heterogeneous 2D layers stacked with a twist angle and/or lattice mismatch. Expanding the range of available materials, methods for fabricating MSL, and realization unique emergent properties key challenges. Here we report facile bottom-up synthesis MSL based on wide-gap semiconductor, BiOCl, using one-pot solvothermal approach robust reproducibility. Unlike previous MSLs usually prepared by directly...

10.1038/s41467-019-12347-7 article EN cc-by Nature Communications 2019-10-02

Achieving large-sized and thinly layered 2D metal phosphorus trichalcogenides with high quality yield has been an urgent quest due to extraordinary physical/chemical characteristics for multiple applications. Nevertheless, current preparation methodologies suffer from uncontrolled thicknesses, uneven morphologies area distributions, long processing times, inferior quality. Here, a sonication-free fast (in minutes) electrochemical cathodic exfoliation approach is reported that can prepare...

10.1002/smll.201902427 article EN Small 2019-06-07

The ingenious surface and electronic structures endow the ultrathin wrinkle-free Pd<sub>4</sub>Cu<sub>1</sub>nanosheets with enhanced methanol oxidation performance.

10.1039/c8ta01912f article EN Journal of Materials Chemistry A 2018-01-01
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